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@ARTICLE{Frankenstein:1024746,
      author       = {Frankenstein, Lars and Mohrhardt, Marvin and Peschel,
                      Christoph and Stolz, Lukas and Gomez-Martin, Aurora and
                      Placke, Tobias and Hur, Hyuck and Winter, Martin and
                      Kasnatscheew, Johannes},
      title        = {{E}xperimental {C}onsiderations of the {C}hemical
                      {P}relithiation {P}rocess via {L}ithium {A}rene {C}omplex
                      {S}olutions on the {E}xample of {S}i‐{B}ased {A}nodes for
                      {L}ithium‐{I}on {B}atteries},
      journal      = {Advanced energy $\&$ sustainability research},
      volume       = {5},
      number       = {2},
      issn         = {2699-9412},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2024-02412},
      pages        = {2300177},
      year         = {2024},
      note         = {Unterstützt durch Grand: SeNSE (no. 875548)},
      abstract     = {Losses of Li inventory in lithium-ion batteries lead to
                      losses in capacity and can be compensated by electrode
                      prelithiation before cell assembly or before cell formation.
                      The approach of chemical prelithiation, for example, via Li
                      arene complex (LAC)-based solutions is technically an
                      apparently simple and promising approach. Nevertheless, as
                      shown herein on the example of Si-based anodes and LAC
                      solutions based on 4,4′-dimethylbiphenyl (4,4′-DMBP),
                      several practical challenges need to be considered. Given
                      their reactivity, the LAC solution can not only decompose
                      itself within a range of a few hours, as seen by
                      discoloration and confirmed via mass spectrometry, but can
                      also decompose its solvent and binder of added composite
                      electrodes. Effective prelithiation requires an excess in
                      capacity of the LAC solution (relative to anode capacity)
                      and optimized system characteristic conditions (time,
                      temperature, etc.) as exemplarily shown by comparing
                      Si-based nanoparticles with nanowires. It is worth noting
                      that the prelithiation degree alone does not determine the
                      boost in cycle life, but relevantly depends on previously
                      applied prelithiation conditions (e.g., temperature), as
                      well.},
      cin          = {IEK-12},
      ddc          = {333.7},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:001109881500001},
      doi          = {10.1002/aesr.202300177},
      url          = {https://juser.fz-juelich.de/record/1024746},
}