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@ARTICLE{Knne:1024778,
      author       = {Künne, Sven and Hesper, Jakob Michael and Lein, Tobias and
                      Voigt, Karsten and Mikhailova, Daria and Michaelis,
                      Alexander and Winter, Martin and Placke, Tobias and Heubner,
                      Christian},
      title        = {{H}ybrid {H}igh‐{V}oltage {L}i{N}i 0.5 {M}n 1.5 {O} 4
                      /{G}raphite {C}athodes {E}nabling {R}echargeable {B}atteries
                      with {S}imultaneous {A}nion‐ and {C}ation {S}torage},
      journal      = {Batteries $\&$ supercaps},
      volume       = {6},
      number       = {9},
      issn         = {2566-6223},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2024-02444},
      pages        = {e202300284},
      year         = {2023},
      note         = {Unterstützt durch den Grant: “GrEEn”(313-W044A)},
      abstract     = {A hybrid cathode concept that targets combining the
                      specific advantages of Li-ion batteries and dual-ion
                      batteries is proposed. LiNi0.5Mn1.5O4 (LNMO), (de)inserting
                      Li+, and graphite, capable to (de)intercalate PF6− present
                      in the electrolyte, are combined in one cathode, aiming for
                      synergy effects due to the presence of two electrochemically
                      active species to overcome rate limitations caused by
                      electrolyte depletion. Hybrid cathodes of different
                      compositions and designs are prepared and investigated
                      regarding their properties and the storage mechanism using
                      electrochemical analyses combined with operando XRD and
                      extensive materials characterization, including scanning
                      electron microscopy and energy-dispersive X-ray
                      spectroscopy. Finally, hybrid cathodes with higher areal
                      capacity are prepared and investigated regarding rate
                      performance. Model-based analysis of the results reveals
                      design criteria and material properties required to achieve
                      synergistic effects between the components in hybrid
                      cathodes. These insights lay the foundation for a new type
                      of battery with advantageous properties in terms of cost,
                      environmental friendliness, and electrochemical
                      performance.},
      cin          = {IEK-12},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:001039746300001},
      doi          = {10.1002/batt.202300284},
      url          = {https://juser.fz-juelich.de/record/1024778},
}