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001024801 1001_ $$0P:(DE-HGF)0$$aWu, Yan$$b0$$eCorresponding author
001024801 245__ $$aCombining Janus Separator and Organic Cathode for Dendrite‐Free and High‐Performance Na‐Organic Batteries
001024801 260__ $$aWeinheim$$bWiley-VCH$$c2024
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001024801 520__ $$aThe growth of Na-dendrites and the dissolution of organic cathodes are twomajor challenges that hinder the development of sodium-organic batteries(SOBs). Herein, a multifunctional Janus separator (h-BN@PP@C) by using aninterfacial engineering strategy, is proposed to tackle the issues of SOBs. Thecarbon layer facing the organic cathode serves as a barrier to capturedissolved organic materials and enhance their utilization. Meanwhile, theh-BN layer facing the Na anode possesses high thermal conductivity andmechanical strength, which mitigates the occurrence of localized-temperature“hot spots” and promotes the formation of a NaF-enriched SEI, therebysuppressing dendrite growth. Consequently, the Janus separator enables astable Na plating/stripping cycling for 1000 h at 3 mA cm−2. Equipped withthe Janus separator, organic cathodes including dibenzo[b,i]thianthrene-5,7,12,14-tetraone (DTT), pentacene-5,7,12,14-tetrone andCalix[4]quinone cathodes demonstrate high capacity and remarkable cyclingperformance. In particular, the DTT exhibits a bipolar co-reaction storagemechanism and achieves an ultrahigh capacity (≈342.6 mAh g−1), long-termcycling stability (capacity decay rate of 0.15% per cycle over 550 cycles at500 mA g−1) and fast kinetics (1000 mA g−1≈2.8 C). This study offers astraightforward, effective, and promising solution to address the challenges in SOBs.
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001024801 7001_ $$0P:(DE-HGF)0$$aWang, Xingchao$$b1
001024801 7001_ $$0P:(DE-HGF)0$$aZhang, Fei$$b2
001024801 7001_ $$0P:(DE-HGF)0$$aHai, Lijuan$$b3
001024801 7001_ $$0P:(DE-HGF)0$$aChen, QiHua$$b4
001024801 7001_ $$0P:(DE-HGF)0$$aChao, Cuiqin$$b5
001024801 7001_ $$0P:(DE-Juel1)180575$$aYang, Aikai$$b6
001024801 7001_ $$0P:(DE-HGF)0$$aSun, Ying$$b7$$eCorresponding author
001024801 7001_ $$0P:(DE-HGF)0$$aJia, Dianzeng$$b8$$eCorresponding author
001024801 773__ $$0PERI:(DE-600)2039420-2$$a10.1002/adfm.202309552$$gVol. 34, no. 8, p. 2309552$$n8$$p2309552$$tAdvanced functional materials$$v34$$x1616-301X$$y2024
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