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| 001 | 1024801 | ||
| 005 | 20250204113829.0 | ||
| 024 | 7 | _ | |a 10.1002/adfm.202309552 |2 doi |
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| 024 | 7 | _ | |a 1099-0712 |2 ISSN |
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| 100 | 1 | _ | |a Wu, Yan |0 P:(DE-HGF)0 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Combining Janus Separator and Organic Cathode for Dendrite‐Free and High‐Performance Na‐Organic Batteries |
| 260 | _ | _ | |a Weinheim |c 2024 |b Wiley-VCH |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 520 | _ | _ | |a The growth of Na-dendrites and the dissolution of organic cathodes are twomajor challenges that hinder the development of sodium-organic batteries(SOBs). Herein, a multifunctional Janus separator (h-BN@PP@C) by using aninterfacial engineering strategy, is proposed to tackle the issues of SOBs. Thecarbon layer facing the organic cathode serves as a barrier to capturedissolved organic materials and enhance their utilization. Meanwhile, theh-BN layer facing the Na anode possesses high thermal conductivity andmechanical strength, which mitigates the occurrence of localized-temperature“hot spots” and promotes the formation of a NaF-enriched SEI, therebysuppressing dendrite growth. Consequently, the Janus separator enables astable Na plating/stripping cycling for 1000 h at 3 mA cm−2. Equipped withthe Janus separator, organic cathodes including dibenzo[b,i]thianthrene-5,7,12,14-tetraone (DTT), pentacene-5,7,12,14-tetrone andCalix[4]quinone cathodes demonstrate high capacity and remarkable cyclingperformance. In particular, the DTT exhibits a bipolar co-reaction storagemechanism and achieves an ultrahigh capacity (≈342.6 mAh g−1), long-termcycling stability (capacity decay rate of 0.15% per cycle over 550 cycles at500 mA g−1) and fast kinetics (1000 mA g−1≈2.8 C). This study offers astraightforward, effective, and promising solution to address the challenges in SOBs. |
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| 700 | 1 | _ | |a Wang, Xingchao |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Zhang, Fei |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Hai, Lijuan |0 P:(DE-HGF)0 |b 3 |
| 700 | 1 | _ | |a Chen, QiHua |0 P:(DE-HGF)0 |b 4 |
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| 700 | 1 | _ | |a Sun, Ying |0 P:(DE-HGF)0 |b 7 |e Corresponding author |
| 700 | 1 | _ | |a Jia, Dianzeng |0 P:(DE-HGF)0 |b 8 |e Corresponding author |
| 773 | _ | _ | |a 10.1002/adfm.202309552 |g Vol. 34, no. 8, p. 2309552 |0 PERI:(DE-600)2039420-2 |n 8 |p 2309552 |t Advanced functional materials |v 34 |y 2024 |x 1616-301X |
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