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001024809 1001_ $$0P:(DE-HGF)0$$aWu, Miaomiao$$b0
001024809 245__ $$aLong-Life Aqueous Zinc–Organic Batteries with a Trimethyl Phosphate Electrolyte and Organic Cathode
001024809 260__ $$aWashington, DC$$bACS Publ.$$c2023
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001024809 520__ $$aAqueous zinc batteries (AZBs) are environment-friendly batteries with good application prospects. However, their applications are plagued by the dendrite growth of Zn anodes and the absence of suitable cathodes. Herein, we design and realize high-performance AZBs by using an organic cathode of 5,7,12,14-pentacenetetrone (PT) and a trimethyl phosphate (TMP)/water hybrid electrolyte. The COMSOL simulations and spectroscopy studies collectively demonstrate a strong interaction between TMP and Zn2+, thus changing the solvation structure and suppressing the parasitic reactions, finally enabling dendrite-free Zn plating/stripping. The hybrid electrolyte shows good compatibility with the PT cathode. As a consequence, the Zn//PT full cell employing the hybrid electrolyte exhibits remarkable capacity (229.4 mA h g–1 at 0.1 A g–1), extraordinary rate performance, and long-term cycling (84.18% retention after 9600 cycles) at a wide temperature range (−20 to 65 °C).
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001024809 7001_ $$0P:(DE-HGF)0$$aSu, Wenqi$$b1
001024809 7001_ $$0P:(DE-HGF)0$$aWang, Xingchao$$b2$$eCorresponding author
001024809 7001_ $$0P:(DE-HGF)0$$aLiu, Zhibo$$b3
001024809 7001_ $$0P:(DE-HGF)0$$aZhang, Fei$$b4
001024809 7001_ $$0P:(DE-HGF)0$$aLuo, Zhiqiang$$b5
001024809 7001_ $$0P:(DE-Juel1)180575$$aYang, Aikai$$b6$$ufzj
001024809 7001_ $$0P:(DE-HGF)0$$aYeleken, Palizhaye$$b7
001024809 7001_ $$0P:(DE-HGF)0$$aMiao, Zezhong$$b8
001024809 7001_ $$0P:(DE-HGF)0$$aHuang, Yudai$$b9
001024809 773__ $$0PERI:(DE-600)2695697-4$$a10.1021/acssuschemeng.2c05410$$gVol. 11, no. 3, p. 957 - 964$$n3$$p957 - 964$$tACS sustainable chemistry & engineering$$v11$$x2168-0485$$y2023
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