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@ARTICLE{vonHoltum:1024885,
      author       = {von Holtum, Bastian and Kubot, Maximilian and Peschel,
                      Christoph and Rodehorst, Uta and Winter, Martin and Nowak,
                      Sascha and Wiemers-Meyer, Simon},
      title        = {{A}ccessing the {P}rimary {S}olid–{E}lectrolyte
                      {I}nterphase on {L}ithium {M}etal: {A} {M}ethod for
                      {L}ow‐{C}oncentration {C}ompound {A}nalysis},
      journal      = {ChemSusChem},
      volume       = {16},
      number       = {9},
      issn         = {1864-5631},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2024-02536},
      pages        = {e202300451},
      year         = {2023},
      abstract     = {Despite large research efforts in the fields of lithium ion
                      and lithium metal batteries, there are still unanswered
                      questions. One of them is the formation of the
                      solid−electrolyte interphase (SEI) in
                      lithium-metal-anode-based battery systems. Until now, a
                      compound profile analysis of the SEI on lithium metal was
                      challenging as the amounts of many compounds after simple
                      contact of lithium metal and the electrolyte were too low
                      for detection with analytical methods. This study presents a
                      novel approach on unravelling the SEI compound profile
                      through accumulation in the gas, liquid electrolyte, and
                      solid phase. The method uses the intrinsic behavior of
                      lithium metal to spontaneously react with the liquid
                      electrolyte. In combination with complementary,
                      state-of-the-art analytical instrumentation and methods,
                      this approach provides qualitative and quantitative results
                      on all three phases revealing the vast variety of compounds
                      formed in carbonate-based electrolytes.},
      cin          = {IEK-12},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122) / Lillint -
                      Thermodynamic and kinetic stability of the Lithium-Liquid
                      Electrolyte Interface (13XP0225C)},
      pid          = {G:(DE-HGF)POF4-1221 / G:(BMBF)13XP0225C},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {37104827},
      UT           = {WOS:000975677100001},
      doi          = {10.1002/cssc.202300451},
      url          = {https://juser.fz-juelich.de/record/1024885},
}