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@ARTICLE{Adhitama:1024888,
      author       = {Adhitama, Egy and Bela, Marlena M. and Demelash, Feleke and
                      Stan, Marian C. and Winter, Martin and Gomez-Martin, Aurora
                      and Placke, Tobias},
      title        = {{O}n the {P}ractical {A}pplicability of the {L}i
                      {M}etal‐{B}ased {T}hermal {E}vaporation {P}relithiation
                      {T}echnique on {S}i {A}nodes for {L}ithium {I}on
                      {B}atteries},
      journal      = {Advanced energy materials},
      volume       = {13},
      number       = {3},
      issn         = {1614-6832},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2024-02539},
      pages        = {2203256},
      year         = {2023},
      note         = {Zudem unterstützt durch BMBF Grant ProLiFest (03XP0253A)},
      abstract     = {Lithium ion batteries (LIBs) using silicon as anode
                      material are endowed with much higher energy density than
                      state-of-the-art graphite-based LIBs. However, challenges of
                      volume expansion and related dynamic surfaces lead to
                      continuous (re-)formation of the solid electrolyte
                      interphase, active lithium losses, and rapid capacity
                      fading. Cell failure can be further accelerated when Si is
                      paired with high-capacity, but also rather reactive Ni-rich
                      cathodes, such as LiNi0.8Co0.1Mn0.1O2 (NCM-811). Here, the
                      practical applicability of thermal evaporation of Li metal
                      is evaluated as a prelithiation technique on
                      micrometer-sized Si (µ-Si) electrodes in addressing such
                      challenges. NCM-811 || “prelithiated µ-Si” full-cells
                      $(25\%$ degree of prelithiation) can attain a higher initial
                      discharge capacity of ≈192 mAh gNCM-811−1 than the cells
                      without prelithiation with only ≈160 mAh gNCM-811−1.
                      This study deeply discusses significant consequences of
                      electrode capacity balancing (N:P ratio) with regard to
                      prelithiation on the performance of full-cells. The
                      trade-off between cell lifetime and energy density is also
                      highlighted. It is essential to point out that the phenomena
                      discussed here can further guide the direction of research
                      in using the thermal evaporation of Li metal as a
                      prelithiation technique toward its practical application on
                      Si-based LIBs.},
      cin          = {IEK-12},
      ddc          = {050},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122) / BACCARA -
                      Battery and superCapacitor ChARActerization and testing
                      (608491)},
      pid          = {G:(DE-HGF)POF4-1221 / G:(EU-Grant)608491},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000891051000001},
      doi          = {10.1002/aenm.202203256},
      url          = {https://juser.fz-juelich.de/record/1024888},
}