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001024903 1001_ $$0P:(DE-HGF)0$$aGöldner, Valentin$$b0
001024903 245__ $$aLaser desorption/ionization-mass spectrometry for the analysis of interphases in lithium ion batteries
001024903 260__ $$aSt. Louis$$bElsevier$$c2023
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001024903 520__ $$aLaser desorption/ionization-mass spectrometry (LDI-MS) is introduced as a complementary technique for the analysis of interphases formed at electrode|electrolyte interfaces in lithium ion batteries (LIBs). An understanding of these interphases is crucial for designing interphase-forming electrolyte formulations and increasing battery lifetime. Especially organic species are analyzed more effectively using LDI-MS than with established methodologies. The combination with trapped ion mobility spectrometry and tandem mass spectrometry yields additional structural information of interphase components. Furthermore, LDI-MS imaging reveals the lateral distribution of compounds on the electrode surface. Using the introduced methods, a deeper understanding of the mechanism of action of the established solid electrolyte interphase-forming electrolyte additive 3,4-dimethyloxazolidine-2,5-dione (Ala-N-CA) for silicon/graphite anodes is obtained, and active electrochemical transformation products are unambiguously identified. In the future, LDI-MS will help to provide a deeper understanding of interfacial processes in LIBs by using it in a multimodal approach with other surface analysis methods to obtain complementary information.
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001024903 7001_ $$0P:(DE-HGF)0$$aQuach, Linda$$b1
001024903 7001_ $$0P:(DE-HGF)0$$aAdhitama, Egy$$b2
001024903 7001_ $$0P:(DE-HGF)0$$aBehrens, Arne$$b3
001024903 7001_ $$0P:(DE-HGF)0$$aJunk, Luisa$$b4
001024903 7001_ $$0P:(DE-Juel1)166130$$aWinter, Martin$$b5$$ufzj
001024903 7001_ $$0P:(DE-HGF)0$$aPlacke, Tobias$$b6
001024903 7001_ $$0P:(DE-HGF)0$$aGlorius, Frank$$b7
001024903 7001_ $$00000-0002-1774-6787$$aKarst, Uwe$$b8$$eCorresponding author
001024903 773__ $$0PERI:(DE-600)2927064-9$$a10.1016/j.isci.2023.107517$$gVol. 26, no. 9, p. 107517 -$$n9$$p107517 -$$tiScience$$v26$$x2589-0042$$y2023
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