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@ARTICLE{Gldner:1024903,
      author       = {Göldner, Valentin and Quach, Linda and Adhitama, Egy and
                      Behrens, Arne and Junk, Luisa and Winter, Martin and Placke,
                      Tobias and Glorius, Frank and Karst, Uwe},
      title        = {{L}aser desorption/ionization-mass spectrometry for the
                      analysis of interphases in lithium ion batteries},
      journal      = {iScience},
      volume       = {26},
      number       = {9},
      issn         = {2589-0042},
      address      = {St. Louis},
      publisher    = {Elsevier},
      reportid     = {FZJ-2024-02553},
      pages        = {107517 -},
      year         = {2023},
      abstract     = {Laser desorption/ionization-mass spectrometry (LDI-MS) is
                      introduced as a complementary technique for the analysis of
                      interphases formed at electrode|electrolyte interfaces in
                      lithium ion batteries (LIBs). An understanding of these
                      interphases is crucial for designing interphase-forming
                      electrolyte formulations and increasing battery lifetime.
                      Especially organic species are analyzed more effectively
                      using LDI-MS than with established methodologies. The
                      combination with trapped ion mobility spectrometry and
                      tandem mass spectrometry yields additional structural
                      information of interphase components. Furthermore, LDI-MS
                      imaging reveals the lateral distribution of compounds on the
                      electrode surface. Using the introduced methods, a deeper
                      understanding of the mechanism of action of the established
                      solid electrolyte interphase-forming electrolyte additive
                      3,4-dimethyloxazolidine-2,5-dione (Ala-N-CA) for
                      silicon/graphite anodes is obtained, and active
                      electrochemical transformation products are unambiguously
                      identified. In the future, LDI-MS will help to provide a
                      deeper understanding of interfacial processes in LIBs by
                      using it in a multimodal approach with other surface
                      analysis methods to obtain complementary information.},
      cin          = {IEK-12},
      ddc          = {050},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {37636078},
      UT           = {WOS:001147801100001},
      doi          = {10.1016/j.isci.2023.107517},
      url          = {https://juser.fz-juelich.de/record/1024903},
}