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| 001 | 1024903 | ||
| 005 | 20250203103204.0 | ||
| 024 | 7 | _ | |a 10.1016/j.isci.2023.107517 |2 doi |
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| 100 | 1 | _ | |a Göldner, Valentin |0 P:(DE-HGF)0 |b 0 |
| 245 | _ | _ | |a Laser desorption/ionization-mass spectrometry for the analysis of interphases in lithium ion batteries |
| 260 | _ | _ | |a St. Louis |c 2023 |b Elsevier |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 336 | 7 | _ | |a Journal Article |0 0 |2 EndNote |
| 520 | _ | _ | |a Laser desorption/ionization-mass spectrometry (LDI-MS) is introduced as a complementary technique for the analysis of interphases formed at electrode|electrolyte interfaces in lithium ion batteries (LIBs). An understanding of these interphases is crucial for designing interphase-forming electrolyte formulations and increasing battery lifetime. Especially organic species are analyzed more effectively using LDI-MS than with established methodologies. The combination with trapped ion mobility spectrometry and tandem mass spectrometry yields additional structural information of interphase components. Furthermore, LDI-MS imaging reveals the lateral distribution of compounds on the electrode surface. Using the introduced methods, a deeper understanding of the mechanism of action of the established solid electrolyte interphase-forming electrolyte additive 3,4-dimethyloxazolidine-2,5-dione (Ala-N-CA) for silicon/graphite anodes is obtained, and active electrochemical transformation products are unambiguously identified. In the future, LDI-MS will help to provide a deeper understanding of interfacial processes in LIBs by using it in a multimodal approach with other surface analysis methods to obtain complementary information. |
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| 700 | 1 | _ | |a Quach, Linda |0 P:(DE-HGF)0 |b 1 |
| 700 | 1 | _ | |a Adhitama, Egy |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Behrens, Arne |0 P:(DE-HGF)0 |b 3 |
| 700 | 1 | _ | |a Junk, Luisa |0 P:(DE-HGF)0 |b 4 |
| 700 | 1 | _ | |a Winter, Martin |0 P:(DE-Juel1)166130 |b 5 |u fzj |
| 700 | 1 | _ | |a Placke, Tobias |0 P:(DE-HGF)0 |b 6 |
| 700 | 1 | _ | |a Glorius, Frank |0 P:(DE-HGF)0 |b 7 |
| 700 | 1 | _ | |a Karst, Uwe |0 0000-0002-1774-6787 |b 8 |e Corresponding author |
| 773 | _ | _ | |a 10.1016/j.isci.2023.107517 |g Vol. 26, no. 9, p. 107517 - |0 PERI:(DE-600)2927064-9 |n 9 |p 107517 - |t iScience |v 26 |y 2023 |x 2589-0042 |
| 856 | 4 | _ | |y OpenAccess |u https://juser.fz-juelich.de/record/1024903/files/Laser%20desorption_ionization-mass%20spectrometry%20for%20the%20analysis%20of%20interphases%20in%20lithium%20ion%20batteries.pdf |
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| 856 | 4 | _ | |y OpenAccess |x icon-180 |u https://juser.fz-juelich.de/record/1024903/files/Laser%20desorption_ionization-mass%20spectrometry%20for%20the%20analysis%20of%20interphases%20in%20lithium%20ion%20batteries.jpg?subformat=icon-180 |
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