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@ARTICLE{Adhitama:1024911,
      author       = {Adhitama, Egy and Refino, Andam Deatama and Brake, Tobias
                      and Pleie, Jan and Schmidt, Christina and Demelash, Feleke
                      and Neuhaus, Kerstin and Bornemann, Steffen and
                      Wiemers-Meyer, Simon and Peiner, Erwin and Winter, Martin
                      and Wasisto, Hutomo Suryo and Placke, Tobias},
      title        = {{O}n the direct correlation between the copper current
                      collector surface area and ‘dead {L}i’ formation in
                      zero-excess {L}i metal batteries},
      journal      = {Journal of materials chemistry / A},
      volume       = {11},
      number       = {14},
      issn         = {2050-7488},
      address      = {London ˜[u.a.]œ},
      publisher    = {RSC},
      reportid     = {FZJ-2024-02561},
      pages        = {7724 - 7734},
      year         = {2023},
      abstract     = {In ‘zero-excess’ (often called ‘anode-free’)
                      lithium metal batteries (ZE-LMBs), three-dimensional (3D)
                      current collectors (CC) with a high surface area have been
                      reported to effectively reduce the local current density and
                      minimize the electronically and/or ionically isolated Li
                      metal, so-called ‘dead Li’. In most of the published
                      works on 3D CCs for ZE-LMBs, the discussion has oftentimes
                      primarily emphasized the relationship between the
                      functionality of the 3D surface structure and its effect on
                      enhanced electrochemical performance. Therefore, it is
                      important to take a deeper look at this relationship by
                      controlling the surface features and surface chemistry of
                      CCs. In this work, the direct correlation between the
                      surface area of CCs and ‘dead Li’ is thoroughly
                      evaluated. The Li deposition behavior at the entire CC is
                      also elucidated. A fair comparison is maintained by
                      precisely controlling surface features and surface chemistry
                      of the 3D copper CC which is realized by
                      femtosecond-laser-ablation. ‘Dead Li’ is accurately
                      quantified by gas chromatography coupled with a barrier
                      discharge ionization detector. This study shall shed light
                      on a deeper understanding of the correlation between surface
                      area and ‘dead Li’ to pave the way for the application
                      of ZE-LMBs.},
      cin          = {IEK-12},
      ddc          = {530},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122) / BACCARA -
                      Battery and superCapacitor ChARActerization and testing
                      (608491)},
      pid          = {G:(DE-HGF)POF4-1221 / G:(EU-Grant)608491},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000955095100001},
      doi          = {10.1039/D3TA00097D},
      url          = {https://juser.fz-juelich.de/record/1024911},
}