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@ARTICLE{Tomar:1024914,
author = {Tomar, Anubha and Adhitama, Egy and Winter, Martin and
Placke, Tobias and Rai, Alok Kumar},
title = {{I}nsights in {U}tilizing {N}i{C}o 2 {O} 4 /{C}o 3 {O} 4
{N}anowires as {A}node {M}aterial in {L}ithium‐{I}on
{B}atteries},
journal = {Batteries $\&$ supercaps},
volume = {6},
number = {3},
issn = {2566-6223},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2024-02564},
pages = {e202200465},
year = {2023},
abstract = {In this study, a facile and cost-effective hydrothermal
approach is employed to synthesize a mesoporous
NiCo2O4/Co3O4 nanocomposite with nanowire morphology by
using polyvinyl pyrrolidone as structure-directing agent.
The obtained NiCo2O4/Co3O4 nanocomposite shows better
electrochemical performance than pure NiCo2O4 due to mainly
two reasons: i) a strong synergistic effect between NiCo2O4
and Co3O4, which enhances the Li+ diffusion rate as well as
lower the charge-transfer resistance, and ii) the
involvement of Co3O4 to contribute to the total capacity due
to its high electrochemical activity. However, the
performance of a NiCo2O4/Co3O4 nanocomposite electrode
starts degrading after 400 cycles while pure NiCo2O4
maintains steady performance. Since the NiCo2O4/Co3O4
nanocomposite sample shows high porosity, it is believed
that the obtained nanowire morphology cannot tolerate volume
variations, which are generally triggered off during
repeated Li+ (de-)insertion at long-term cycling. Therefore,
the obtained results bring new insights in terms that there
is a sweet spot between Li+ diffusion and high porosity in
utilizing Co3O4 within a nanocomposite. This study is of
guidance to shed the light on the research of ternary
transition metal oxide nanocomposite materials for
lithium-ion batteries.},
cin = {IEK-12},
ddc = {540},
cid = {I:(DE-Juel1)IEK-12-20141217},
pnm = {1221 - Fundamentals and Materials (POF4-122) / BACCARA -
Battery and superCapacitor ChARActerization and testing
(608491)},
pid = {G:(DE-HGF)POF4-1221 / G:(EU-Grant)608491},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000907979400001},
doi = {10.1002/batt.202200465},
url = {https://juser.fz-juelich.de/record/1024914},
}