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@ARTICLE{Wasylowski:1024925,
author = {Wasylowski, David and Neubauer, Sven and Faber, Matthias
and Ditler, Heinrich and Sonnet, Morian and Blömeke,
Alexander and Dechent, Philipp and Gitis, Alexander and
Sauer, Dirk Uwe},
title = {{I}n situ tomography of lithium-ion battery cells enabled
by scanning acoustic imaging},
journal = {Journal of power sources},
volume = {580},
issn = {0378-7753},
address = {New York, NY [u.a.]},
publisher = {Elsevier},
reportid = {FZJ-2024-02575},
pages = {233295 -},
year = {2023},
note = {Zudem unterstützt durch BMBF Grants: MADAM4Life (grant
number 03XP0327C), NUBase (grant number 03XP0322C)},
abstract = {Imaging the interior of battery cells provides vital
information for battery manufacturing, as well as lifetime
and performance prediction. This work demonstrates a
scalable and in-situ method to image the structural state of
battery cells with layer resolution. Building on our prior
publication, we apply ultrasound waves on pouch cells and
process the reflected instead of the transmitted wave. This
allows us to utilize time-of-flight data to provide depth
information for later signal parts. We develop and
demonstrate an algorithm that dissects the reflected
ultrasound wave and calculates individual reflections from
material interfaces within the electrode stack by fitting
their estimated envelopes onto the Hilbert transformation of
the entire wave. Consecutive individual reflections are used
to calculate the reflection coefficient from the material
interface, which is then mapped onto a color map. Using this
algorithm, we image an aged and pristine pouch cell from the
same manufacturing batch. The generated images showed a
clear correlation with optical images from a post-mortem
analysis. Indications from the ultrasound image were
verified as lithium-plating.},
cin = {IEK-12},
ddc = {620},
cid = {I:(DE-Juel1)IEK-12-20141217},
pnm = {1223 - Batteries in Application (POF4-122) / InOPlaBat -
In-Situ und Operando Plating Detektion in Batterien
(13XP0352B)},
pid = {G:(DE-HGF)POF4-1223 / G:(BMBF)13XP0352B},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001024330300001},
doi = {10.1016/j.jpowsour.2023.233295},
url = {https://juser.fz-juelich.de/record/1024925},
}