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001024926 1001_ $$00000-0001-9829-0971$$aRefino, Andam Deatama$$b0$$eCorresponding author
001024926 245__ $$aImpact of exposing lithium metal to monocrystalline vertical silicon nanowires for lithium-ion microbatteries
001024926 260__ $$aLondon$$bSpringer Nature$$c2023
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001024926 500__ $$aZudem unterstützt durch BMBF Projekt: ProLiFest (03XP0253A)
001024926 520__ $$aSilicon has attracted considerable attention for use as high-capacity anodes of lithium-ion microbatteries. However, its extreme volume change upon (de-)lithiation still poses a challenge for adoption as it leads to severe active lithium loss that shortens the cycle life. Here, we fabricate three-dimensional monocrystalline vertical silicon nanowires on a silicon wafer using low-cost metal-assisted chemical etching, then cover them with lithium using thermal evaporation prior to the battery operation as the pre-lithiation step, to investigate its impact on electrochemical performance. To reveal the underlying physical and electrochemical mechanisms, we also process a comparative planar monocrystalline silicon. We find that pre-lithiation results in improved (de-)lithiation behavior, especially in planar silicon-based cells, while silicon nanowire-based cells exhibit low capacity in early cycles. This study sheds light on the surface design and structural modification of monocrystalline silicon nanowires with respect to pre-lithiation by lithium thermal evaporation.
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001024926 7001_ $$00000-0002-7637-1356$$aAdhitama, Egy$$b1
001024926 7001_ $$0P:(DE-HGF)0$$aBela, Marlena M.$$b2
001024926 7001_ $$0P:(DE-HGF)0$$aSadhujan, Sumesh$$b3
001024926 7001_ $$0P:(DE-HGF)0$$aHarilal, Sherina$$b4
001024926 7001_ $$00000-0001-6414-3658$$aEldona, Calvin$$b5
001024926 7001_ $$aBremers, Heiko$$b6
001024926 7001_ $$00000-0002-0371-7088$$aBashouti, Muhammad Y.$$b7
001024926 7001_ $$aSumboja, Afriyanti$$b8
001024926 7001_ $$aStan, Marian C.$$b9
001024926 7001_ $$0P:(DE-Juel1)166130$$aWinter, Martin$$b10
001024926 7001_ $$00000-0002-2097-5193$$aPlacke, Tobias$$b11
001024926 7001_ $$aPeiner, Erwin$$b12
001024926 7001_ $$00000-0002-4522-3625$$aWasisto, Hutomo Suryo$$b13
001024926 773__ $$0PERI:(DE-600)3008524-X$$a10.1038/s43246-023-00385-0$$gVol. 4, no. 1, p. 58$$n1$$p58$$tCommunications materials$$v4$$x2662-4443$$y2023
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