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| 001 | 1024926 | ||
| 005 | 20250203103402.0 | ||
| 024 | 7 | _ | |a 10.1038/s43246-023-00385-0 |2 doi |
| 024 | 7 | _ | |a 10.34734/FZJ-2024-02576 |2 datacite_doi |
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| 037 | _ | _ | |a FZJ-2024-02576 |
| 082 | _ | _ | |a 600 |
| 100 | 1 | _ | |a Refino, Andam Deatama |0 0000-0001-9829-0971 |b 0 |e Corresponding author |
| 245 | _ | _ | |a Impact of exposing lithium metal to monocrystalline vertical silicon nanowires for lithium-ion microbatteries |
| 260 | _ | _ | |a London |c 2023 |b Springer Nature |
| 336 | 7 | _ | |a article |2 DRIVER |
| 336 | 7 | _ | |a Output Types/Journal article |2 DataCite |
| 336 | 7 | _ | |a Journal Article |b journal |m journal |0 PUB:(DE-HGF)16 |s 1712747914_24399 |2 PUB:(DE-HGF) |
| 336 | 7 | _ | |a ARTICLE |2 BibTeX |
| 336 | 7 | _ | |a JOURNAL_ARTICLE |2 ORCID |
| 336 | 7 | _ | |a Journal Article |0 0 |2 EndNote |
| 500 | _ | _ | |a Zudem unterstützt durch BMBF Projekt: ProLiFest (03XP0253A) |
| 520 | _ | _ | |a Silicon has attracted considerable attention for use as high-capacity anodes of lithium-ion microbatteries. However, its extreme volume change upon (de-)lithiation still poses a challenge for adoption as it leads to severe active lithium loss that shortens the cycle life. Here, we fabricate three-dimensional monocrystalline vertical silicon nanowires on a silicon wafer using low-cost metal-assisted chemical etching, then cover them with lithium using thermal evaporation prior to the battery operation as the pre-lithiation step, to investigate its impact on electrochemical performance. To reveal the underlying physical and electrochemical mechanisms, we also process a comparative planar monocrystalline silicon. We find that pre-lithiation results in improved (de-)lithiation behavior, especially in planar silicon-based cells, while silicon nanowire-based cells exhibit low capacity in early cycles. This study sheds light on the surface design and structural modification of monocrystalline silicon nanowires with respect to pre-lithiation by lithium thermal evaporation. |
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| 536 | _ | _ | |a BACCARA - Battery and superCapacitor ChARActerization and testing (608491) |0 G:(EU-Grant)608491 |c 608491 |f FP7-ENERGY-2013-1 |x 1 |
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| 700 | 1 | _ | |a Adhitama, Egy |0 0000-0002-7637-1356 |b 1 |
| 700 | 1 | _ | |a Bela, Marlena M. |0 P:(DE-HGF)0 |b 2 |
| 700 | 1 | _ | |a Sadhujan, Sumesh |0 P:(DE-HGF)0 |b 3 |
| 700 | 1 | _ | |a Harilal, Sherina |0 P:(DE-HGF)0 |b 4 |
| 700 | 1 | _ | |a Eldona, Calvin |0 0000-0001-6414-3658 |b 5 |
| 700 | 1 | _ | |a Bremers, Heiko |b 6 |
| 700 | 1 | _ | |a Bashouti, Muhammad Y. |0 0000-0002-0371-7088 |b 7 |
| 700 | 1 | _ | |a Sumboja, Afriyanti |b 8 |
| 700 | 1 | _ | |a Stan, Marian C. |b 9 |
| 700 | 1 | _ | |a Winter, Martin |0 P:(DE-Juel1)166130 |b 10 |
| 700 | 1 | _ | |a Placke, Tobias |0 0000-0002-2097-5193 |b 11 |
| 700 | 1 | _ | |a Peiner, Erwin |b 12 |
| 700 | 1 | _ | |a Wasisto, Hutomo Suryo |0 0000-0002-4522-3625 |b 13 |
| 773 | _ | _ | |a 10.1038/s43246-023-00385-0 |g Vol. 4, no. 1, p. 58 |0 PERI:(DE-600)3008524-X |n 1 |p 58 |t Communications materials |v 4 |y 2023 |x 2662-4443 |
| 856 | 4 | _ | |y OpenAccess |u https://juser.fz-juelich.de/record/1024926/files/Impact%20of%20exposing%20lithium%20metal%20to%20monocrystalline%20vertical%20silicon%20nanowires%20for%20lithium-ion%20microbatteries.pdf |
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