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@ARTICLE{Wrogemann:1025009,
      author       = {Wrogemann, Jens Matthies and Lüther, Marco Joes and
                      Bärmann, Peer and Lounasvuori, Mailis and Javed, Ali and
                      Tiemann, Michael and Golnak, Ronny and Xiao, Jie and Petit,
                      Tristan and Placke, Tobias and Winter, Martin},
      title        = {{O}vercoming {D}iffusion {L}imitation of {F}aradaic
                      {P}rocesses: {P}roperty‐{P}erformance {R}elationships of
                      2{D} {C}onductive {M}etal‐{O}rganic {F}ramework {C}u 3
                      ({HHTP}) 2 for {R}eversible {L}ithium‐{I}on {S}torage},
      journal      = {Angewandte Chemie},
      volume       = {62},
      number       = {26},
      issn         = {1433-7851},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2024-02603},
      pages        = {e202303111},
      year         = {2023},
      note         = {Gefördert durch MWIDE NRW “GrEEn”(313-W044A),},
      abstract     = {Faradaic reactions including charge transfer are often
                      accompanied with diffusion limitation inside the bulk.
                      Conductive two-dimensional frameworks (2D MOFs) with a fast
                      ion transport can combine both—charge transfer and fast
                      diffusion inside their porous structure. To study remaining
                      diffusion limitations caused by particle morphology,
                      different synthesis routes of
                      Cu-2,3,6,7,10,11-hexahydroxytriphenylene (Cu3(HHTP)2), a
                      copper-based 2D MOF, are used to obtain flake- and rod-like
                      MOF particles. Both morphologies are systematically
                      characterized and evaluated for redox-active Li+ ion
                      storage. The redox mechanism is investigated by means of
                      X-ray absorption spectroscopy, FTIR spectroscopy and in situ
                      XRD. Both types are compared regarding kinetic properties
                      for Li+ ion storage via cyclic voltammetry and impedance
                      spectroscopy. A significant influence of particle morphology
                      for 2D MOFs on kinetic aspects of electrochemical Li+ ion
                      storage can be observed. This study opens the path for
                      optimization of redox active porous structures to overcome
                      diffusion limitations of Faradaic processes.},
      cin          = {IEK-12},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {37069123},
      UT           = {WOS:000989585400001},
      doi          = {10.1002/anie.202303111},
      url          = {https://juser.fz-juelich.de/record/1025009},
}