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| Hauptseite > Publikationsdatenbank > Monitoring the Formation of Nickel-Poor and Nickel-Rich Oxide Cathode Materials for Lithium-Ion Batteries with Synchrotron Radiation > print |
| Hauptseite > Publikationsdatenbank > Monitoring the Formation of Nickel-Poor and Nickel-Rich Oxide Cathode Materials for Lithium-Ion Batteries with Synchrotron Radiation > print |
| 001 | 1025011 | ||
| 005 | 20250203103250.0 | ||
| 024 | 7 | _ | |a 10.1021/acs.chemmater.2c02639 |2 doi |
| 024 | 7 | _ | |a 0897-4756 |2 ISSN |
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| 037 | _ | _ | |a FZJ-2024-02605 |
| 082 | _ | _ | |a 540 |
| 100 | 1 | _ | |a Ying, Bixian |b 0 |
| 245 | _ | _ | |a Monitoring the Formation of Nickel-Poor and Nickel-Rich Oxide Cathode Materials for Lithium-Ion Batteries with Synchrotron Radiation |
| 260 | _ | _ | |a Washington, DC |c 2023 |b American Chemical Society |
| 336 | 7 | _ | |a article |2 DRIVER |
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| 336 | 7 | _ | |a Journal Article |b journal |m journal |0 PUB:(DE-HGF)16 |s 1712752390_24402 |2 PUB:(DE-HGF) |
| 336 | 7 | _ | |a ARTICLE |2 BibTeX |
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| 500 | _ | _ | |a Unterstützt durch BMBF Projekt: 03XP0231 |
| 520 | _ | _ | |a The syntheses of Ni-poor (NCM111, LiNi1/3Co1/3Mn1/3O2) and Ni-rich (NCM811 LiNi0.8Co0.1Mn0.1O2) lithium transition-metal oxides (space group R3̅m) from hydroxide precursors (Ni1/3Co1/3Mn1/3(OH)2, Ni0.8Co0.1Mn0.1(OH)2) are investigated using in situ synchrotron powder diffraction and near-edge X-ray absorption fine structure spectroscopy. The development of the layered structure of these two cathode materials proceeds via two utterly different reaction mechanisms. While the synthesis of NCM811 involves a rock salt-type intermediate phase, NCM111 reveals a layered structure throughout the entire synthesis. Moreover, the necessity and the impact of a preannealing step and a high-temperature holding step are discussed. |
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| 700 | 1 | _ | |a Fitzpatrick, Jack R. |0 0000-0003-4704-9242 |b 1 |
| 700 | 1 | _ | |a Teng, Zhenjie |b 2 |
| 700 | 1 | _ | |a Chen, Tianxiang |b 3 |
| 700 | 1 | _ | |a Lo, Tsz Woon Benedict |b 4 |
| 700 | 1 | _ | |a Siozios, Vassilios |b 5 |
| 700 | 1 | _ | |a Murray, Claire A. |0 0000-0002-8306-3634 |b 6 |
| 700 | 1 | _ | |a Brand, Helen E. A. |b 7 |
| 700 | 1 | _ | |a Day, Sarah |b 8 |
| 700 | 1 | _ | |a Tang, Chiu C. |b 9 |
| 700 | 1 | _ | |a Weatherup, Robert S. |0 0000-0002-3993-9045 |b 10 |
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| 700 | 1 | _ | |a Schuppler, Stefan |0 P:(DE-HGF)0 |b 13 |
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| 700 | 1 | _ | |a Kleiner, Karin |0 0000-0003-0203-440X |b 15 |e Corresponding author |
| 773 | _ | _ | |a 10.1021/acs.chemmater.2c02639 |g Vol. 35, no. 4, p. 1514 - 1526 |0 PERI:(DE-600)1500399-1 |n 4 |p 1514 - 1526 |t Chemistry of materials |v 35 |y 2023 |x 0897-4756 |
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