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| Hauptseite > Publikationsdatenbank > Multiple protective layers for suppressing Li dendrite growth and improving the cycle life of anode-free lithium metal batteries > print |
| Hauptseite > Publikationsdatenbank > Multiple protective layers for suppressing Li dendrite growth and improving the cycle life of anode-free lithium metal batteries > print |
| 001 | 1025019 | ||
| 005 | 20240712113105.0 | ||
| 024 | 7 | _ | |a 10.1016/j.cej.2024.149547 |2 doi |
| 024 | 7 | _ | |a 1385-8947 |2 ISSN |
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| 024 | 7 | _ | |a 1873-3212 |2 ISSN |
| 024 | 7 | _ | |a 1873-5541 |2 ISSN |
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| 037 | _ | _ | |a FZJ-2024-02613 |
| 100 | 1 | _ | |a Merso, Semaw Kebede |b 0 |
| 245 | _ | _ | |a Multiple protective layers for suppressing Li dendrite growth and improving the cycle life of anode-free lithium metal batteries |
| 260 | _ | _ | |a Amsterdam |c 2024 |b Elsevier |
| 336 | 7 | _ | |a article |2 DRIVER |
| 336 | 7 | _ | |a Output Types/Journal article |2 DataCite |
| 336 | 7 | _ | |a Journal Article |b journal |m journal |0 PUB:(DE-HGF)16 |s 1712826126_17869 |2 PUB:(DE-HGF) |
| 336 | 7 | _ | |a ARTICLE |2 BibTeX |
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| 336 | 7 | _ | |a Journal Article |0 0 |2 EndNote |
| 520 | _ | _ | |a Anode-free lithium metal batteries (AFLMBs) have sparked considerable attention in recent years because of their potential for high energy density; however, they suffer from severe Li dendrite growth and unstable solid electrolyte interphase (SEI), which typically result in rapid capacity decay. Herein, we demonstrate a long-life anode-free pouch cell by designing a dual-coating protective layer (Cu-Sn@SFPH) electrode with Sn-coated Cu (denoted as Cu-Sn) as the bottom layer and SrF2 nanoparticles strengthened by poly (vinylidene fluoride)-co-hexafluoropropylene (PVDF-HFP) as the top layer. The in-situ formed LiF-rich SEI enables fast Li+ transfer, while the lithiophilic Li-Sn and Li-Sr alloy layers serve as nucleation seeds for uniform Li deposition. The dual-coated Cu electrode in the Cu-Sn@SFPH||Li cell exhibits remarkable cycling stability for more than 3,200 h at a capacity of 2 mAh cm−2. The NCM111||Cu-Sn@SFPH pouch cell demonstrates outstanding performance with a capacity retention of 72.1 % and an average Coulombic efficiency (CE) of 99.9 % for 120 cycles. Under practical conditions, with NCM cathodes and a lean electrolyte volume, this design strategy opens a new approach to AFLMBs. |
| 536 | _ | _ | |a 1221 - Fundamentals and Materials (POF4-122) |0 G:(DE-HGF)POF4-1221 |c POF4-122 |f POF IV |x 0 |
| 536 | _ | _ | |a LiBEST2 - Lithium-Batterie-Konzepte mit hoher Energiedichte, Leistung und Sicherheit (13XP0304A) |0 G:(BMBF)13XP0304A |c 13XP0304A |x 1 |
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| 700 | 1 | _ | |a Tekaligne, Teshager Mekonnen |b 1 |
| 700 | 1 | _ | |a Adigo Weret, Misganaw |b 2 |
| 700 | 1 | _ | |a Shitaw, Kassie Nigus |b 3 |
| 700 | 1 | _ | |a Nikodimos, Yosef |0 0000-0002-2929-3965 |b 4 |
| 700 | 1 | _ | |a Yang, Sheng-Chiang |b 5 |
| 700 | 1 | _ | |a Muche, Zabish Bilew |b 6 |
| 700 | 1 | _ | |a Taklu, Bereket Woldegbreal |b 7 |
| 700 | 1 | _ | |a Hotasi, Boas Tua |b 8 |
| 700 | 1 | _ | |a Chang, Chia-Yu |0 P:(DE-HGF)0 |b 9 |
| 700 | 1 | _ | |a Jiang, Shi-Kai |0 P:(DE-HGF)0 |b 10 |
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| 700 | 1 | _ | |a Winter, Martin |0 P:(DE-Juel1)166130 |b 12 |
| 700 | 1 | _ | |a Wu, She-Huang |0 0000-0003-1165-9444 |b 13 |
| 700 | 1 | _ | |a Su, Wei-Nien |0 0000-0003-1494-2675 |b 14 |
| 700 | 1 | _ | |a Mou, Chung-Yuan |b 15 |
| 700 | 1 | _ | |a Hwang, Bing Joe |0 P:(DE-Juel1)188933 |b 16 |e Corresponding author |
| 773 | _ | _ | |a 10.1016/j.cej.2024.149547 |g Vol. 485, p. 149547 - |0 PERI:(DE-600)2012137-4 |p 149547 - |t The chemical engineering journal |v 485 |y 2024 |x 1385-8947 |
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