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@ARTICLE{Li:1025221,
      author       = {Li, Cheng-Feng and Muruganantham, Rasu and Hsu, Wei-Chun
                      and Ihrig, Martin and Hsieh, Chien-Te and Wang, Chih-Chieh
                      and Liu, Wei-Ren},
      othercontributors = {Finsterbusch, Martin},
      title        = {{A}tomic layer deposition of {Z}n{O} on
                      {L}i1.3{A}l0.3{T}i1.7({PO}4)3 enables its application in all
                      solid-state lithium batteries},
      journal      = {Journal of the Taiwan Institute of Chemical Engineers},
      volume       = {144},
      issn         = {1876-1070},
      address      = {Amsterdam [u.a.]},
      publisher    = {Elsevier},
      reportid     = {FZJ-2024-02789},
      pages        = {104681 -},
      year         = {2023},
      abstract     = {BackgroundAll-solid-state Li batteries (ASSLBs) are
                      emerging as potential electrochemical energy storage devices
                      for next-generation large-scale electrical power systems. In
                      particular, Li1.3Al0.3Ti1.7(PO4)3 (LATP) is an efficient
                      cost-effective solid-state electrolyte with high ionic
                      conductivity for high energy density and safety ASSLBs.
                      Since LATP is unstable verus metallic Li. Therefore, the
                      application of Li-based all-solid-state batteries is
                      practically limited.MethodsAs a possible solution to
                      overcome the LATP instability, the interface was modified by
                      adding a 5 nm thin ZnO layer on LATP using the atomic layer
                      deposition (ALD) technique.Significant FindingsThe ZnO layer
                      reduces the observed overpotential in a Li|ZnO@LATP|Li
                      symmetric cell compared to an unmodified LATP-based cell. In
                      contrast to the unmodified LATP-based Li cells, the
                      ZnO-modified symmetric LATP-based Li cells show stable
                      cycling for more than 500 h without a short circuit. The
                      full-cell configuration of the LiFePO4|ZnO@LATP|Li system
                      showed a reversible capacity of 156 mAh/g over 50 cycles and
                      exposed good capacity retention $(98.79\%$ after 50 cycles)
                      during the cycling test. The results indicate that ZnO
                      coating by ALD on LATP could overcome the stability issues
                      of pristine LATP versus metallic Li. Therefore, this work
                      will lead to prove the simple manner of interfacial
                      modification and improvement of electrochemical performance
                      of inorganic oxide based solid electrolytes for
                      all-solid-state lithium battery applications.},
      cin          = {IEK-1},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-1-20101013},
      pnm          = {1221 - Fundamentals and Materials (POF4-122) / 1222 -
                      Components and Cells (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221 / G:(DE-HGF)POF4-1222},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000946520900001},
      doi          = {10.1016/j.jtice.2023.104681},
      url          = {https://juser.fz-juelich.de/record/1025221},
}