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@ARTICLE{Schomburg:1025925,
      author       = {Schomburg, Felix and Heidrich, Bastian and Wennemar, Sarah
                      and Drees, Robin and Roth, Thomas and Kurrat, Michael and
                      Heimes, Heiner and Jossen, Andreas and Winter, Martin and
                      Cheong, Jun Young and Röder, Fridolin},
      title        = {{L}ithium-ion battery cell formation: status and future
                      directions towards a knowledge-based process design},
      journal      = {Energy $\&$ environmental science},
      volume       = {17},
      number       = {8},
      issn         = {1754-5692},
      address      = {Cambridge},
      publisher    = {RSC Publ.},
      reportid     = {FZJ-2024-03203},
      pages        = {2686 - 2733},
      year         = {2024},
      note         = {Zudem unterstützt durch das Projekt "FormEL’’
                      (03XP0296E) als Teil des Kompetenzklusters ProZell’’ des
                      BMBF.},
      abstract     = {The battery cell formation is one of the most critical
                      process steps in lithium-ion battery (LIB) cell production,
                      because it affects the key battery performance metrics, e.g.
                      rate capability, lifetime and safety, is time-consuming and
                      contributes significantly to energy consumption during cell
                      production and overall cell cost. As LIBs usually exceed the
                      electrochemical sability window of the electrolyte,
                      formation is required to activate and stabilise the
                      electrochemical reactions. Enhanced battery technologies are
                      poised to further expand voltage windows and harness
                      conversion or metal electrodes to elevate energy density,
                      thereby magnifying the significance of cell formation in the
                      battery realm. Despite its critical importance, even the
                      understanding of the formation process of conventional LIBs
                      is still incomplete due to numerous influencing factors.
                      Complex internal processes and the associated high
                      experimental and simulation effort make it difficult to gain
                      a thorough understanding of the process and hence to
                      optimise it. This review paper provides a systematic
                      overview of the formation process and its influencing
                      factors. It is emphasized that material and cell design and
                      the formation process are not independent, but must
                      interlock with each other. Promising experimental and
                      simulative methods to gain the required understanding of the
                      interplay for a truly knowledge-based design of the
                      formation process are highlighted. In the concluding
                      discussion research gaps are identified and a perspective
                      for development of tailored cell formation processes for
                      current and future battery technologies is outlined.},
      cin          = {IEK-12},
      ddc          = {690},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122) / DFG project
                      533115776 - Enthüllung der mikrostrukturellen und
                      elektrochemischen Entwicklung einer
                      Si/Sn-Nanofaserverbundanode für Lithium-Ionen-Batterien
                      (533115776)},
      pid          = {G:(DE-HGF)POF4-1221 / G:(GEPRIS)533115776},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:001166413700001},
      doi          = {10.1039/D3EE03559J},
      url          = {https://juser.fz-juelich.de/record/1025925},
}