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@ARTICLE{Desmaizieres:1025930,
author = {Desmaizieres, Gauthier and Perner, Verena and Wassy, Daniel
and Kolek, Martin and Bieker, Peter and Winter, Martin and
Esser, Birgit},
title = {{E}valuating the {P}olymer {B}ackbone – {V}inylene versus
{S}tyrene – of {A}nisyl‐substituted {P}henothiazines as
{B}attery {E}lectrode {M}aterials},
journal = {Batteries $\&$ supercaps},
volume = {6},
number = {2},
issn = {2566-6223},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2024-03208},
pages = {e202200464},
year = {2023},
abstract = {Organic electrode materials are capable candidates for
next-generation greener energy storage solutions. One
advantage is that their electrochemical performance can be
tuned by structural modification. We herein investigate
anisyl-substituted poly(vinyl-) and
poly(styrylphenothiazines) as positive electrode materials
for dual-ion batteries. π-Interactions – characteristic
to phenothiazine redox polymers – are facilitated in the
poly(styrene) derivatives PSAPT and PSAPT-X-DVB due to the
longer spacing between phenothiazine units and polymer
backbone and lead to high cycling stabilities, but reduce
their specific capacities. In the poly(vinylenes), the
linear PVAPT shows high cycling stability but a
dissolution/redeposition mechanism, diminishing its
capacity, while the cross-linked X-PVAPT demonstrates high
cycling stabilities at specific capacities up to
81 mAh g−1 paired with an excellent rate performance,
where 10,000 cycles at 100 C rate proceed with $86 \%$
capacity retention.},
cin = {IEK-12},
ddc = {540},
cid = {I:(DE-Juel1)IEK-12-20141217},
pnm = {1221 - Fundamentals and Materials (POF4-122) / DFG project
230408635 - Entwicklung organischer Materialien zur
Energiespeicherung, für elektrooptische Anwendungen und als
Template für neuartige Nanoröhren (230408635) / DFG
project 398214985 - Heteroaromatische Redoxpolymere für
Lithium-/organische Batterien (HALO) (398214985) / DFG
project 390874152 - EXC 2154: POLiS - Post Lithium Storage
Cluster of Excellence (390874152)},
pid = {G:(DE-HGF)POF4-1221 / G:(GEPRIS)230408635 /
G:(GEPRIS)398214985 / G:(GEPRIS)390874152},
typ = {PUB:(DE-HGF)16},
UT = {WOS:000905832600001},
doi = {10.1002/batt.202200464},
url = {https://juser.fz-juelich.de/record/1025930},
}