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@ARTICLE{nal:1026942,
      author       = {Ünal, Leyla and Maccio-Figgemeier, Viviane and
                      Gebresilassie Eshetu, Gebrekidan and Figgemeier, Egbert},
      title        = {{I}n‐{V}itro {E}lectrochemical {P}relithiation: {A} {K}ey
                      {P}erformance‐{B}oosting {S}trategy for {C}arbon
                      {N}anotube‐{C}ontaining {S}ilicon‐{B}ased {N}egative
                      {E}lectrodes in {L}i‐{I}on {B}atteries},
      journal      = {ChemElectroChem},
      volume       = {11},
      number       = {17},
      issn         = {2196-0216},
      address      = {Weinheim},
      publisher    = {Wiley-VCH},
      reportid     = {FZJ-2024-03534},
      pages        = {e202400146},
      year         = {2024},
      note         = {The authors acknowledge the Federal Ministry of Education
                      and Research of Germany (BMBF) for funding this work through
                      the projects, PräLi (03XP0238X) and ProMIZ (13XP0397B).
                      Open-Access funding enabled and organized by Projekt DEAL.},
      abstract     = {Prelithiation technology has emerged as an enabling
                      approach towards the practical deployment of Silicon
                      negative electrode-based Li-Ion batteries, leading to
                      significant advancement in initial Coulombic efficiency
                      (ICE), energy density and cycle life. In this study, an
                      electrochemical prelithiation has been applied to
                      Multi-Walled Carbon Nanotubes (MWCNTs)-containing
                      Silicon-rich Silicon/Graphite-based negative electrode,
                      eliminating almost $~51.03 \%$ of its first irreversible
                      capacity losses. In contrast, a benchmarking negative
                      electrode utilizing Carbon black (Super P) as conductive
                      additive is found to demonstrate a reduction of
                      $~39.55 \%$ after prelithiation, which is considerably
                      lower compared to MWCNTs-based electrode system. Post-mortem
                      analysis using Energy-dispersive X-ray (EDX) analysis with a
                      Scanning Electron Microscope (SEM) and Attenuated Total
                      Reflection Fourier Transform Infrared Spectroscopy
                      (ATR-FTIR) shows disparities between pristine-cycled and
                      prelithiated-cycled negative electrodes. Overall,
                      prelithiation enabled MWCNTs can be regarded as an essential
                      additive component in Silicon-based negative electrode
                      systems for high-energy density Li-Ion batteries.},
      cin          = {IEK-12},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IEK-12-20141217},
      pnm          = {1221 - Fundamentals and Materials (POF4-122)},
      pid          = {G:(DE-HGF)POF4-1221},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:001234783100001},
      doi          = {10.1002/celc.202400146},
      url          = {https://juser.fz-juelich.de/record/1026942},
}