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001027281 1001_ $$0P:(DE-Juel1)181018$$aKrämer, S.$$b0$$eFirst author
001027281 245__ $$aTeaching an old dog new tricks: Ti-doped ZnFe 2 O 4 as active material in zinc ion batteries – a proof of concept
001027281 260__ $$aBeijing$$bRoyal Society of Chemistry$$c2024
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001027281 520__ $$aIn this work, the suitability of the spinel material ZnFe2O4, which has already been widely investigated in the context of its magnetic and photocatalytic properties, for use as active material for the cathode side in zinc ion batteries is presented. In addition to pure ZnFe2O4, part of the Fe³⁺ was doped with Ti⁴⁺ to achieve stabilization of Zn vacancies in the material and increase ionic conductivity as indicated by previous modelling results. Ceramic samples with the composition ZnFe2−xTixO4 (x = 0 to 0.25) were prepared via a Pechini synthesis route and investigated regarding their optical, structural and electrochemical characteristics. It has been successfully demonstrated that both pure and Ti doped ZnFe2O4 can be used as active material in the positive electrodes of zinc metal batteries or in an “anode-free” setup with Sn metal. Cells with calcined ZnFe2xTixO4 (x = 0.09)|0.5 M zinc triflate in acetonitrile|Zn showed a stable cycling behavior over 1000 cycles and an average initial specific capacity of 55 mA h g⁻¹.
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001027281 7001_ $$0P:(DE-Juel1)198851$$aHopster, Julia$$b1$$eFirst author
001027281 7001_ $$0P:(DE-Juel1)188297$$aWindmüller, Anna$$b2
001027281 7001_ $$0P:(DE-Juel1)156123$$aEichel, Rüdiger-A.$$b3$$ufzj
001027281 7001_ $$0P:(DE-Juel1)166392$$aGrünebaum, M.$$b4
001027281 7001_ $$00000-0002-9455-5044$$aJüstel, T.$$b5
001027281 7001_ $$0P:(DE-Juel1)166130$$aWinter, M.$$b6
001027281 7001_ $$0P:(DE-Juel1)181017$$aNeuhaus, Kerstin$$b7$$eCorresponding author
001027281 773__ $$0PERI:(DE-600)3168416-6$$a10.1039/D4YA00134F$$gp. 10.1039.D4YA00134F$$n9$$p2175-2185$$tEnergy advances$$v3$$x2753-1457$$y2024
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