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@ARTICLE{Krmer:1027281,
author = {Krämer, S. and Hopster, Julia and Windmüller, Anna and
Eichel, Rüdiger-A. and Grünebaum, M. and Jüstel, T. and
Winter, M. and Neuhaus, Kerstin},
title = {{T}eaching an old dog new tricks: {T}i-doped {Z}n{F}e 2 {O}
4 as active material in zinc ion batteries – a proof of
concept},
journal = {Energy advances},
volume = {3},
number = {9},
issn = {2753-1457},
address = {Beijing},
publisher = {Royal Society of Chemistry},
reportid = {FZJ-2024-03725},
pages = {2175-2185},
year = {2024},
abstract = {In this work, the suitability of the spinel material
ZnFe2O4, which has already been widely investigated in the
context of its magnetic and photocatalytic properties, for
use as active material for the cathode side in zinc ion
batteries is presented. In addition to pure ZnFe2O4, part of
the Fe³⁺ was doped with Ti⁴⁺ to achieve stabilization
of Zn vacancies in the material and increase ionic
conductivity as indicated by previous modelling results.
Ceramic samples with the composition ZnFe2−xTixO4 (x = 0
to 0.25) were prepared via a Pechini synthesis route and
investigated regarding their optical, structural and
electrochemical characteristics. It has been successfully
demonstrated that both pure and Ti doped ZnFe2O4 can be used
as active material in the positive electrodes of zinc metal
batteries or in an “anode-free” setup with Sn metal.
Cells with calcined ZnFe2xTixO4 (x = 0.09)|0.5 M zinc
triflate in acetonitrile|Zn showed a stable cycling behavior
over 1000 cycles and an average initial specific capacity of
55 mA h g⁻¹.},
cin = {IEK-12 / IEK-9},
ddc = {620},
cid = {I:(DE-Juel1)IEK-12-20141217 / I:(DE-Juel1)IEK-9-20110218},
pnm = {1221 - Fundamentals and Materials (POF4-122) / 1222 -
Components and Cells (POF4-122) / 1223 - Batteries in
Application (POF4-122)},
pid = {G:(DE-HGF)POF4-1221 / G:(DE-HGF)POF4-1222 /
G:(DE-HGF)POF4-1223},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001248228000001},
doi = {10.1039/D4YA00134F},
url = {https://juser.fz-juelich.de/record/1027281},
}