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001     1027304
005     20250204113903.0
024 7 _ |a 10.1016/j.carbon.2024.119252
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024 7 _ |a 0008-6223
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024 7 _ |a 1873-3891
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024 7 _ |a 10.34734/FZJ-2024-03735
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037 _ _ |a FZJ-2024-03735
082 _ _ |a 540
100 1 _ |a Fiedler, Magdalena
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245 _ _ |a The role of nanoporous carbon materials for thiophosphate-based all solid state lithium sulfur battery performance
260 _ _ |a Amsterdam [u.a.]
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500 _ _ |a This research and development results are funded by the German Federal Ministry of Education and Research (BMBF) within the SoLiS project (Grant No. 03XP0395) and AReLiS-3 project (03XP0595).
520 _ _ |a Due to their high theoretical energy density, all solid state lithium sulfur batteries (LS-SSB) represent one of the most promising candidates for next-generation energy storage systems. Whilst high sulfur utilizations have been published for several cathode compositions and preparation methods in recent years, there is still a lack of clarity regarding the influence of the used carbon. Furthermore, LS-SSBs face challenges in up-scaling as the common preparation methods including high energy ball milling are time consuming, batch-wise and need high energy impact. In this study, high sulfur utilization >1600 mAh g$_S^{−1}$ and reversibility with 80 % of initial discharge capacity after 60 cycles is achieved, using a more time-efficient preparation method with drastically lowered energy impact by selecting a suitable carbon. Additionally, the influence of the carbon nanostructure on the electrochemical performance is discussed. This study provides guidance in selecting nanostructured carbon materials to enable cost-efficient, up-scalable preparation methods for LS-SSBs without compromising on the excellent electrochemical performance.
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700 1 _ |a Lange, Martin A.
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700 1 _ |a Hippauf, Felix
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700 1 _ |a Dörfler, Susanne
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700 1 _ |a Althues, Holger
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700 1 _ |a Zeier, Wolfgang G.
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700 1 _ |a Kaskel, Stefan
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773 _ _ |a 10.1016/j.carbon.2024.119252
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