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@TECHREPORT{Wilden:1028266,
author = {Wilden, Andreas and Sauerwein, Fynn Sören and Schneider,
Dimitri and Paparigas, Zaina and Henkes, Maximilian and
Vanel, Vincent and Geist, Andreas and Modolo, Giuseppe},
title = {{PATRICIA} {D}eliverable {D}2.3 {E}xperimental
demonstration and validation of a spiked {AMSEL} flowsheet
test},
reportid = {FZJ-2024-04455},
pages = {16 p.},
year = {2024},
abstract = {This document provides the results of an experimental
demonstration and validation of a spiked AMSEL flowsheet
test, which was conducted at FZJ. The AmSEL process uses
TODGA as an extractant and SO3-Ph-BTBP as an Am(III)
selective complexant. The process was run in the 16-stage
centrifugal contactor setup installed in the FZJ
laboratories, using a flowsheet designed and optimised by
CEA. An Am(III) product containing $45\%$ Am(III) with only
$5\%$ Cm(III) contamination was obtained. The remaining
Am(III), Cm(III) and Ln(III) were routed to the spent
solvent. The separation from Ln(III) was very good with high
decontamination factors. However, significant recycling of
Am(III) occurred, which needs to be addressed in further
process optimizations. More centrifugal contactor stages are
required to improve Am(III) recovery and the Am/Cm
decontamination factor.},
cin = {IEK-6},
cid = {I:(DE-Juel1)IEK-6-20101013},
pnm = {1412 - Predisposal (POF4-141) / PATRICIA - Partitioning And
Transmuter Research Initiative in a Collaborative Innovation
Action (945077)},
pid = {G:(DE-HGF)POF4-1412 / G:(EU-Grant)945077},
typ = {PUB:(DE-HGF)15},
url = {https://juser.fz-juelich.de/record/1028266},
}