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024 7 _ |a 10.1063/1.3236529
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100 1 _ |0 P:(DE-Juel1)VDB56587
|a Strozecka, A.
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245 _ _ |a Modification of the conductance of single fullerene molecules by endohedral doping
260 _ _ |a Melville, NY
|b American Institute of Physics
|c 2009
300 _ _ |a 133118
336 7 _ |a Journal Article
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440 _ 0 |0 562
|a Applied Physics Letters
|v 95
|x 0003-6951
|y 13
500 _ _ |a This work was supported by the FP6 project NANO-CAGE (Grant No. MEST-CT-2004-50-6854), the Science Foundation of Ireland, and Czech Project MSM Grant No. 0021620834. We acknowledge the Irish Centre for High-End Computing (ICHEC) for generous allotment of computer resources.
520 _ _ |a We use scanning tunneling microscopy to establish controlled contacts to single molecules of endohedrally doped Ce-2@C-80 fullerenes with C-60 as a reference. The stability of the experimental setup allows for the determination of the conductance of Ce-2@C-80 relative to the conductance of C-60. The endohedral doping reduces the conductance of Ce-2@C-80 by a factor of about five with respect to C-60. Ab initio calculations show that the reason for this reduced conductance is the absence of electron orbitals delocalized over the cage of Ce-2@C-80 in the energy window of the conductance measurement. (C) 2009 American Institute of Physics. [doi:10.1063/1.3236529]
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