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@INPROCEEDINGS{Sarner:1030408,
author = {Sarner, Stephan and Menzler, Norbert H. and Guillon,
Olivier},
title = {{C}losing the {L}oop:{A}dvancing {S}olid {O}xide {C}ell
{C}eramics in the {C}ircular {E}conomy},
reportid = {FZJ-2024-05281},
year = {2024},
abstract = {The adoption of fuel cell and hydrogen technologies will
play a crucial role in facilitating the shift towards
decarbonization and meeting the EU's goal of achieving zero
net greenhouse gas emissions by 2050. In the coming years,
particular emphasis will be placed on expanding the
deployment of suitable hydrogen electrolyzers, such as solid
oxide electrolysis cells (SOECs), which currently have a
moderate technology readiness level (TRL 5-7). To support
market entry and promote resource recovery, early-stage
development and implementation of recycling strategies are
imperative. Efforts are underway to address the reuse and
recovery of components from high-temperature electrolyzers,
focusing on the reprocessing of ceramic components from
End-of-Life solid oxide cells (SOCs). Establishing
closed-loop recycling processes is highly desirable, with a
focus on scalability. In line with this objective, a
recovery route has been devised for the well-established
fuel electrode-supported cell design. The primary goal is to
reprocess more than $80\%$ of the cell material into new
substrate, directly applicable in the SOC device. Therefore,
a prerequisite step involves the separation of the oxygen
electrode and any potential contact layer, which can be
achieved through mechanical and/or hydrometallurgical
approaches. Subsequently, the sintered bodies undergo
reprocessing into ceramic powder, substrate slurry, and
ultimately the pre-sintered substrate. Components of the
separated oxygen electrode are recovered as precursors,
suitable for SOC applications (e.g., manufacturing oxygen
electrodes or contact layers) or alternative uses.In
addition to presenting the properties of the recycled
substrate, full cells were manufactured based on substrates
containing $0\%,$ $25\%,$ and $50\%$ recyclate by weight.
Electrochemical tests were conducted to determine whether
these substrates meet the functional requirements, including
gas distribution, electrical conductivity, and mechanical
stability.},
month = {Aug},
date = {2024-08-19},
organization = {14th International Conference on
Ceramic Materials and Components for
Energy and Environmental Systems,
Budapest (Hungary), 19 Aug 2024 - 22
Aug 2024},
subtyp = {After Call},
cin = {IMD-2},
cid = {I:(DE-Juel1)IMD-2-20101013},
pnm = {1231 - Electrochemistry for Hydrogen (POF4-123) / SOFC -
Solid Oxide Fuel Cell (SOFC-20140602)},
pid = {G:(DE-HGF)POF4-1231 / G:(DE-Juel1)SOFC-20140602},
typ = {PUB:(DE-HGF)6},
url = {https://juser.fz-juelich.de/record/1030408},
}