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001030857 1001_ $$0P:(DE-Juel1)190965$$aZhou, Hangyu$$b0$$eCorresponding author$$ufzj
001030857 245__ $$aKagomerization of transition metal monolayers induced by two-dimensional hexagonal boron nitride
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001030857 520__ $$aThe kagome lattice is an exciting solid state physics platform for the emergence of nontrivial quantum states driven by electronic correlations: topological effects, unconventional superconductivity, charge and spin density waves, and unusual magnetic states such as quantum spin liquids. While kagome lattices have been realized in complex multi-atomic bulk compounds, here we demonstrate from first-principles a process that we dub kagomerization, in which we fabricate a two-dimensional kagome lattice in monolayers of transition metals utilizing an hexagonal boron nitride (h-BN) overlayer. Surprisingly, h-BN induces a large rearrangement of the transition metal atoms supported on a fcc(111) heavy-metal surface. This reconstruction is found to be rather generic for this type of heterostructures and has a profound impact on the underlying magnetic properties, ultimately stabilizing various topological magnetic solitons such as skyrmions and bimerons. Our findings call for a reconsideration of h-BN as merely a passive capping layer, showing its potential for not only reconstructing the atomic structure of the underlying material, e.g. through the kagomerization of magnetic films, but also enabling electronic and magnetic phases that are highly sought for the next generation of device technologies.
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001030857 536__ $$0G:(GEPRIS)462676712$$aDFG project G:(GEPRIS)462676712 - iAFMskyrmionen- Intrinsische antiferromagnetische Skyrmionen aus ersten Prinzipien: Von der Stabilisierung, der Interaktion mit Defekten bis zum effizienten Nachweis (462676712)$$c462676712$$x2
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001030857 7001_ $$0P:(DE-Juel1)145395$$ados Santos Dias, Manuel$$b1$$ufzj
001030857 7001_ $$0P:(DE-HGF)0$$aZhang, Youguang$$b2
001030857 7001_ $$0P:(DE-HGF)0$$aZhao, Weisheng$$b3$$eCorresponding author
001030857 7001_ $$0P:(DE-Juel1)130805$$aLounis, Samir$$b4$$eCorresponding author
001030857 773__ $$0PERI:(DE-600)2553671-0$$a10.1038/s41467-024-48973-z$$gVol. 15, no. 1, p. 4854$$n1$$p4854$$tNature Communications$$v15$$x2041-1723$$y2024
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001030857 9101_ $$0I:(DE-HGF)0$$6P:(DE-Juel1)190965$$a School of Electronic and Information Engineering, Beihang University, Beijing, 100191, China$$b0
001030857 9101_ $$0I:(DE-HGF)0$$6P:(DE-Juel1)190965$$a Fert Beijing Institute, School of Integrated Circuit Science and Engineering, Beihang University, Beijing, 100191, China$$b0
001030857 9101_ $$0I:(DE-HGF)0$$6P:(DE-Juel1)190965$$a Shenyuan Honors College, Beihang University, Beijing, 100191, China$$b0
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001030857 9101_ $$0I:(DE-HGF)0$$6P:(DE-Juel1)145395$$a Scientific Computing Department, STFC Daresbury Laboratory, Warrington, WA4 4AD, United Kingdom$$b1
001030857 9101_ $$0I:(DE-HGF)0$$6P:(DE-Juel1)145395$$a Faculty of Physics, University of Duisburg-Essen and CENIDE, 47053, Duisburg, Germany$$b1
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