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000010311 084__ $$2WoS$$aPhysics, Multidisciplinary
000010311 1001_ $$0P:(DE-HGF)0$$aStadler, C.$$b0
000010311 245__ $$aTuning intermolecular interaction in long-range-ordered submonolayer organic films
000010311 260__ $$aBasingstoke$$bNature Publishing Group$$c2009
000010311 300__ $$a153 - 158
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000010311 440_0 $$014921$$aNature Physics$$v5$$x1745-2473
000010311 500__ $$aWe thank F. Pollinger and the ESRF staff ( T.- L. Lee, J. Zegenhagen) for their help during the XSW experiments. Financial support by the BMBF, the DFG and the ESRF is acknowledged.
000010311 520__ $$aThe future success of organic electronic devices strongly depends on the ability to tailor the properties of thin films and interfaces. This calls for well-ordered thin films. However, their properties are dominantly influenced by the formation of the first molecular layer representing a template for further growth. The development of the first layer-in turn-depends on the fine balance of molecule-substrate and molecule-molecule interaction. The latter is usually attractive owing to van der Waals forces and causes the formation of islands and small crystalline grains. Here, we report on organic adsorbates exhibiting a repulsive intermolecular interaction. With increasing coverage, Sn-phthalocyanine molecules continuously rearrange on Ag(111) in a series of ordered superstructures. They always fill the surface terraces homogeneously and maximize the domain size. Thicker films also exhibit extremely large, monocrystalline grains and potentially enable bulk-like properties for thin films. The intermolecular interaction can be tuned by cooling and becomes attractive below similar to 120 K.
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000010311 7001_ $$0P:(DE-HGF)0$$aHansen, S.$$b1
000010311 7001_ $$0P:(DE-Juel1)VDB93047$$aKröger, I.$$b2$$uFZJ
000010311 7001_ $$0P:(DE-HGF)0$$aUmbach, E.$$b3
000010311 7001_ $$0P:(DE-Juel1)VDB77884$$aKumpf, C.$$b4$$uFZJ
000010311 773__ $$0PERI:(DE-600)2206346-8$$a10.1038/nphys1176$$gVol. 5, p. 153 - 158$$p153 - 158$$q5<153 - 158$$tNature physics$$v5$$x1745-2473$$y2009
000010311 8567_ $$uhttp://dx.doi.org/10.1038/nphys1176
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000010311 9141_ $$y2009
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