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@ARTICLE{Stadler:10311,
      author       = {Stadler, C. and Hansen, S. and Kröger, I. and Umbach, E.
                      and Kumpf, C.},
      title        = {{T}uning intermolecular interaction in long-range-ordered
                      submonolayer organic films},
      journal      = {Nature physics},
      volume       = {5},
      issn         = {1745-2473},
      address      = {Basingstoke},
      publisher    = {Nature Publishing Group},
      reportid     = {PreJuSER-10311},
      pages        = {153 - 158},
      year         = {2009},
      note         = {We thank F. Pollinger and the ESRF staff ( T.- L. Lee, J.
                      Zegenhagen) for their help during the XSW experiments.
                      Financial support by the BMBF, the DFG and the ESRF is
                      acknowledged.},
      abstract     = {The future success of organic electronic devices strongly
                      depends on the ability to tailor the properties of thin
                      films and interfaces. This calls for well-ordered thin
                      films. However, their properties are dominantly influenced
                      by the formation of the first molecular layer representing a
                      template for further growth. The development of the first
                      layer-in turn-depends on the fine balance of
                      molecule-substrate and molecule-molecule interaction. The
                      latter is usually attractive owing to van der Waals forces
                      and causes the formation of islands and small crystalline
                      grains. Here, we report on organic adsorbates exhibiting a
                      repulsive intermolecular interaction. With increasing
                      coverage, Sn-phthalocyanine molecules continuously rearrange
                      on Ag(111) in a series of ordered superstructures. They
                      always fill the surface terraces homogeneously and maximize
                      the domain size. Thicker films also exhibit extremely large,
                      monocrystalline grains and potentially enable bulk-like
                      properties for thin films. The intermolecular interaction
                      can be tuned by cooling and becomes attractive below similar
                      to 120 K.},
      keywords     = {J (WoSType)},
      cin          = {IBN-3 / JARA-FIT},
      ddc          = {530},
      cid          = {I:(DE-Juel1)VDB801 / $I:(DE-82)080009_20140620$},
      pnm          = {Kondensierte Materie},
      pid          = {G:(DE-Juel1)FUEK414},
      shelfmark    = {Physics, Multidisciplinary},
      typ          = {PUB:(DE-HGF)16},
      UT           = {WOS:000263458500021},
      doi          = {10.1038/nphys1176},
      url          = {https://juser.fz-juelich.de/record/10311},
}