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| 001 | 1031177 | ||
| 005 | 20250203133207.0 | ||
| 024 | 7 | _ | |a 10.1002/smll.202404537 |2 doi |
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| 037 | _ | _ | |a FZJ-2024-05581 |
| 082 | _ | _ | |a 620 |
| 100 | 1 | _ | |a Scharf, Felix |0 P:(DE-Juel1)188525 |b 0 |
| 245 | _ | _ | |a Synergistic Enhancement of Mechanical and Electrochemical Properties in Grafted Polymer/Oxide Hybrid Electrolytes |
| 260 | _ | _ | |a Weinheim |c 2024 |b Wiley-VCH |
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| 500 | _ | _ | |a Zudem unterstützt durch: “FB2-Hybrid” (grant: 13XP0428A), “FB2-TheoDat” (grant: 03XP0435A/E). |
| 520 | _ | _ | |a Lithium metal batteries operated with high voltage cathodes are predestined for the realization of high energy storage systems, where solid polymer electrolytes offer a possibility to improve battery safety. Al2O3_PCL is introduced as promising hybrid electrolyte made from polycaprolactone (PCL) and Al2O3 nanoparticles that can be prepared in a one-pot synthesis as a random mixture of linear PCL and PCL-grafted Al2O3. Upon grafting, synergistic effects of mechanical stability and ionic conductivity are achieved. Due to the mechanical stability, manufacture of PCL-based membranes with a thickness of 50 µm is feasible, yielding an ionic conductivity of 5·10−5 S cm−1 at 60 °C. The membrane exhibits an impressive performance of Li deposition in symmetric Li||Li cells, operating for 1200 h at a constant and low overvoltage of 54 mV and a current density of 0.2 mA cm−2. NMC622 | Al2O3_PCL | Li cells are cycled at rates of up to 1 C, achieving 140 cycles at >80% state of health. The straightforward synthesis and opportunity of upscaling as well as solvent-free polymerization render the Al2O3_PCL hybrid material as rather safe, potentially sustainable and affordable alternative to conventional polymer-based electrolytes. |
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| 700 | 1 | _ | |a Krude, Annalena |0 P:(DE-Juel1)194100 |b 1 |u fzj |
| 700 | 1 | _ | |a Lennartz, Peter |0 P:(DE-Juel1)164855 |b 2 |
| 700 | 1 | _ | |a Clausnitzer, Moritz |0 0009-0000-4743-4947 |b 3 |
| 700 | 1 | _ | |a Shukla, Gourav |0 0009-0002-6259-3377 |b 4 |
| 700 | 1 | _ | |a Buchheit, Annika |0 P:(DE-Juel1)180325 |b 5 |
| 700 | 1 | _ | |a Kempe, Fabian |b 6 |
| 700 | 1 | _ | |a Diddens, Diddo |0 P:(DE-Juel1)169877 |b 7 |
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| 700 | 1 | _ | |a Mitchell, Melanie M. |0 P:(DE-Juel1)192389 |b 9 |u fzj |
| 700 | 1 | _ | |a Danner, Timo |0 0000-0003-2336-6059 |b 10 |
| 700 | 1 | _ | |a Heuer, Andreas |0 P:(DE-Juel1)176646 |b 11 |u fzj |
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| 700 | 1 | _ | |a Brunklaus, Gunther |0 P:(DE-Juel1)172047 |b 14 |
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| 856 | 4 | _ | |u https://juser.fz-juelich.de/record/1031177/files/Small%20-%202024%20-%20Scharf%20-%20Synergistic%20Enhancement%20of%20Mechanical%20and%20Electrochemical%20Properties%20in%20Grafted%20Polymer%20Oxide-1.pdf |y OpenAccess |
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