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@ARTICLE{Mozumder:1031812,
author = {Mozumder, Rubel and Wasmer, Johannes and Antognini Silva,
David and Blügel, Stefan and Rüßmann, Philipp},
title = {{H}igh-throughput magnetic co-doping and design of exchange
interactions in a topological insulator},
reportid = {FZJ-2024-05831, arXiv:2407.04413},
year = {2024},
abstract = {Using high-throughput automation of ab-initio impurity
embedding simulations, we created a database of $3d$ and
$4d$ transition metal defects embedded into the prototypical
topological insulator (TI) Bi$_2$Te$_3$. We simulate both
single impurities as well as impurity dimers at different
impurity-impurity distances inside the TI. We extract
changes to magnetic moments, analyze the polarizability of
non-magnetic impurity atoms via nearby magnetic impurity
atoms and calculate the exchange coupling constants for a
Heisenberg Hamiltonian. We uncover chemical trends in the
exchange coupling constants and discuss the impurities'
potential with respect to magnetic order in the fields of
quantum anomalous Hall insulators and topological quantum
computing. In particular, we predict that co-doping of
different magnetic dopants is a viable strategy to engineer
the magnetic ground state in magnetic TIs.},
cin = {PGI-1 / IAS-1},
cid = {I:(DE-Juel1)PGI-1-20110106 / I:(DE-Juel1)IAS-1-20090406},
pnm = {5211 - Topological Matter (POF4-521) / EXC 2004: Matter
and Light for Quantum Computing (ML4Q) (390534769) / AIDAS -
Joint Virtual Laboratory for AI, Data Analytics and Scalable
Simulation $(aidas_20200731)$ / HDS LEE - Helmholtz School
for Data Science in Life, Earth and Energy (HDS LEE)
(HDS-LEE-20190612)},
pid = {G:(DE-HGF)POF4-5211 / G:(BMBF)390534769 /
$G:(DE-Juel-1)aidas_20200731$ /
G:(DE-Juel1)HDS-LEE-20190612},
typ = {PUB:(DE-HGF)25},
eprint = {2407.04413},
howpublished = {arXiv:2407.04413},
archivePrefix = {arXiv},
SLACcitation = {$\%\%CITATION$ = $arXiv:2407.04413;\%\%$},
doi = {10.34734/FZJ-2024-05831},
url = {https://juser.fz-juelich.de/record/1031812},
}