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@ARTICLE{Blum:1031874,
author = {Blum, Volker and Asahi, Ryoji and Autschbach, Jochen and
Bannwarth, Christoph and Bihlmayer, Gustav and Blügel,
Stefan and Burns, Lori A. and Crawford, T. Daniel and
Dawson, William and de Jong, Wibe Albert and Draxl, Claudia
and Filippi, Claudia and Genovese, Luigi and Giannozzi,
Paolo and Govind, Niranjan and Hammes-Schiffer, Sharon and
Hammond, Jeff R. and Hourahine, Benjamin and Jain, Anubhav
and Kanai, Yosuke and Kent, Paul R C and Larsen, Ask Hjorth
and Lehtola, Susi and Li, Xiaosong and Lindh, Roland and
Maeda, Satoshi and Makri, Nancy and Moussa, Jonathan and
Nakajima, Takahito and Nash, Jessica A. and Oliveira, Micael
J. T. and Patel, Pansy D. and Pizzi, Giovanni and Pourtois,
Geoffrey and Pritchard, Benjamin P. and Rabani, Eran and
Reiher, Markus and Reining, Lucia and Ren, Xinguo and Rossi,
Mariana and Schlegel, H. Bernhard and Seriani, Nicola and
Slipchenko, Lyudmila V. and Thom, Alexander and Valeev,
Edward F. and Van Troeye, Benoit and Visscher, Lucas and
Vlcek, Vojtech and Werner, Hans-Joachim and Williams-Young,
David B. and Windus, Theresa},
title = {{R}oadmap on methods and software for electronic structure
based simulations in chemistry and materials},
journal = {Electronic structure},
volume = {6},
number = {4},
issn = {2516-1075},
address = {Philadelphia, PA},
publisher = {IOP Publishing Ltd.},
reportid = {FZJ-2024-05882},
pages = {042501},
year = {2024},
abstract = {This Roadmap article provides a succinct, comprehensive
overview of the state of electronic structure methods and
software for molecular and materials simulations. Seventeen
distinct sections collect insights by 51 leading scientists
in the field. Each contribution addresses the status of a
particular area, as well as current challenges and
anticipated future advances, with a particular eye towards
software related aspects and providing key references for
further reading. Foundational sections cover density
functional theory and its implementation in real-world
simulation frameworks, Green's function based many-body
perturbation theory, wave-function based and stochastic
electronic structure approaches, relativistic effects and
semiempirical electronic structure theory approaches.
Subsequent sections cover nuclear quantum effects, real-time
propagation of the electronic structure, challenges for
computational spectroscopy simulations, and exploration of
complex potential energy surfaces. The final sections
summarize practical aspects, including computational
workflows for complex simulation tasks, the impact of
current and future high-performance computing architectures,
software engineering practices, education and training to
maintain and broaden the community, as well as the status of
and needs for electronic structure based modeling from the
vantage point of industry environments. Overall, the field
of electronic structure software and method development
continues to unlock immense opportunities for future
scientific discovery, based on the growing ability of
computations to reveal complex phenomena, processes and
properties that are determined by the make-up of matter at
the atomic scale, with high precision.},
cin = {PGI-1},
ddc = {621.3},
cid = {I:(DE-Juel1)PGI-1-20110106},
pnm = {5211 - Topological Matter (POF4-521)},
pid = {G:(DE-HGF)POF4-5211},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001374683700001},
doi = {10.1088/2516-1075/ad48ec},
url = {https://juser.fz-juelich.de/record/1031874},
}