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@ARTICLE{Fogh:1033676,
author = {Fogh, Ellen and Nayak, Mithilesh and Prokhnenko, Oleksandr
and Bartkowiak, Maciej and Munakata, Koji and Soh, Jian-Rui
and Turrini, Alexandra A. and Zayed, Mohamed E. and
Pomjakushina, Ekaterina and Kageyama, Hiroshi and Nojiri,
Hiroyuki and Kakurai, Kazuhisa and Normand, Bruce and Mila,
Frédéric and Rønnow, Henrik M.},
title = {{F}ield-induced bound-state condensation and spin-nematic
phase in {S}r{C}u2({BO}3)2 revealed by neutron scattering up
to 25.9 {T}},
journal = {Nature Communications},
volume = {15},
number = {1},
issn = {2041-1723},
address = {[London]},
publisher = {Nature Publishing Group UK},
reportid = {FZJ-2024-06538},
pages = {442},
year = {2024},
abstract = {In quantum magnetic materials, ordered phases induced by an
applied magnetic field can be described as the Bose-Einstein
condensation (BEC) of magnon excitations. In the strongly
frustrated system SrCu2(BO3)2, no clear magnon BEC could be
observed, pointing to an alternative mechanism, but the high
fields required to probe this physics have remained a
barrier to detailed investigation. Here we exploit the first
purpose-built high-field neutron scattering facility to
measure the spin excitations of SrCu2(BO3)2 up to 25.9 T and
use cylinder matrix-product-states (MPS) calculations to
reproduce the experimental spectra with high accuracy.
Multiple unconventional features point to a condensation of
S = 2 bound states into a spin-nematic phase, including the
gradients of the one-magnon branches and the persistence of
a one-magnon spin gap. This gap reflects a direct analogy
with superconductivity, suggesting that the spin-nematic
phase in SrCu2(BO3)2 is best understood as a condensate of
bosonic Cooper pairs.},
cin = {JCNS-FRM-II / MLZ},
ddc = {500},
cid = {I:(DE-Juel1)JCNS-FRM-II-20110218 / I:(DE-588b)4597118-3},
pnm = {632 - Materials – Quantum, Complex and Functional
Materials (POF4-632) / 6G4 - Jülich Centre for Neutron
Research (JCNS) (FZJ) (POF4-6G4) / HERO - Hidden, entangled
and resonating orders (810451)},
pid = {G:(DE-HGF)POF4-632 / G:(DE-HGF)POF4-6G4 /
G:(EU-Grant)810451},
experiment = {EXP:(DE-MLZ)PANDA-20140101},
typ = {PUB:(DE-HGF)16},
pubmed = {38200029},
UT = {WOS:001141040600024},
doi = {10.1038/s41467-023-44115-z},
url = {https://juser.fz-juelich.de/record/1033676},
}