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@ARTICLE{Bhandari:1034171,
author = {Bhandari, Sabita and Eichel, Rüdiger-A. and Luna, Ana
Laura and Mechler, Anna Katharina},
collaboration = {Schierholz, Roland},
title = {{E}xploring the {E}ffect of {B}all {M}illing on the
{P}hysicochemical {P}roperties and {O}xygen {E}volution
{R}eaction {A}ctivity of {N}ickel and {C}obalt {O}xides},
journal = {Advanced energy $\&$ sustainability research},
volume = {5},
number = {12},
issn = {2699-9412},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2024-06982},
pages = {2400183},
year = {2024},
abstract = {Ball milling is commonly used to reduce catalyst particle
size. However, littleattention is paid to further changes
that ball milling can cause to the rest of thecatalysts’
physicochemical properties, which can impact their intrinsic
catalyticactivity. The effect of ball milling on the
physicochemical properties of NiCoO2 ,NiO, CoO, and NiO:CoO
mixtures is reported and correlated with their
elec-trochemical oxygen evolution reaction (OER) activity.
It is also shown thatparticle fragmentation is an inherent
consequence of ball milling, but someoxides can also
experience a phase transformation. In the case of
rocksalt-structured CoO, it is partially or entirely
transformed to spinel-structuredCo 3O 4 . Additionally, NiCo
2O 4 with a spinel structure can be formed by ballmilling
NiO and CoO simultaneously (both rocksalt structures), but
only in theabsence of water. The changes impact the
electrochemical activity of the initialoxides. Ball milled
NiCoO 2 exhibits the highest activity with a mean
potentialof 1.563 V at 10 mA cm2 , demonstrating the
advantage of having Ni and Co inthe same structure. Although
NiCo2O4 is also a binary oxide, the results indicatethat its
metal coordination environment makes it intrinsically less
active thanNiCoO2 for the OER in alkaline media..},
cin = {IET-1},
ddc = {333.7},
cid = {I:(DE-Juel1)IET-1-20110218},
pnm = {1231 - Electrochemistry for Hydrogen (POF4-123)},
pid = {G:(DE-HGF)POF4-1231},
typ = {PUB:(DE-HGF)16},
UT = {WOS:001328530600001},
doi = {10.1002/aesr.202400183},
url = {https://juser.fz-juelich.de/record/1034171},
}