001034174 001__ 1034174 001034174 005__ 20250203133242.0 001034174 0247_ $$2doi$$a10.1002/smll.202408044 001034174 0247_ $$2ISSN$$a1613-6810 001034174 0247_ $$2ISSN$$a1613-6829 001034174 0247_ $$2datacite_doi$$a10.34734/FZJ-2024-06985 001034174 0247_ $$2pmid$$a39584382 001034174 0247_ $$2WOS$$aWOS:001362082500001 001034174 037__ $$aFZJ-2024-06985 001034174 082__ $$a620 001034174 1001_ $$0P:(DE-HGF)0$$aKnispel, Timo$$b0 001034174 245__ $$aEngineering 2D Materials from Single‐Layer NbS 2 001034174 260__ $$aWeinheim$$bWiley-VCH$$c2025 001034174 3367_ $$2DRIVER$$aarticle 001034174 3367_ $$2DataCite$$aOutput Types/Journal article 001034174 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1738235099_29871 001034174 3367_ $$2BibTeX$$aARTICLE 001034174 3367_ $$2ORCID$$aJOURNAL_ARTICLE 001034174 3367_ $$00$$2EndNote$$aJournal Article 001034174 520__ $$aStarting from a single layer of NbS2 grown on graphene by molecular beam epitaxy, the single unit cell thick 2D materials Nb5/3S3-2D and Nb2S3-2D are created using two different pathways. Either annealing under sulfur-deficient conditions at progressively higher temperatures or deposition of increasing amounts of Nb at elevated temperature result in phase-pure Nb5/3S3-2D followed by Nb2S3-2D. The materials are characterized by scanning tunneling microscopy, scanning tunneling spectroscopy, and X-ray photoemission spectroscopy. The experimental assessment combined with systematic density functional theory calculations reveals their structure. The 2D materials are covalently bound without any van der Waals gap. 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