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001035293 1001_ $$0P:(DE-Juel1)179050$$aThienenkamp, Johannes H.$$b0$$eCorresponding author
001035293 245__ $$aExperimental correlation of anionic mass transport and lithium dendrite growth in solid-state polymer-based lithium metal batteries
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001035293 520__ $$aVarious metal deposition models have been proposed for alkali metal batteries, but the experimental acces-sibility of designated driving forces and characteristics of specific morphologies is still limited. A combinedmethod portfolio comprising operando 1D 19 F MRI, in situ 7 Li NMR, and dynamic electrochemical impedancespectroscopy (EIS) experiments is presented. Experimental evidence of the relation of capacity-degradingdendritic Li metal growth and anionic mass-transport quantities beyond Sand’s time in polymer-based Limetal batteries is demonstrated. Comparison of anionic mass transport and morphological changes in Limetal in Li||Li and NMC 622||Li cells revealed that elevated anion drift velocities within electrolytes are corre-lated with pronounced dendrite growth. Higher cell voltages are associated with increased anion drift veloc-ities and hence dendrite growth, as reflected by a 2.5-fold increase in velocities in NMC 622||Li compared to Li||Li cells. This highlights the potential of the introduced method portfolio for experimental evaluation of poly-mer electrolytes and artificial coatings suitable for alkali metal batteries
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001035293 7001_ $$0P:(DE-Juel1)164855$$aLennartz, Peter$$b1
001035293 7001_ $$0P:(DE-Juel1)166130$$aWinter, Martin$$b2
001035293 7001_ $$0P:(DE-Juel1)172047$$aBrunklaus, Gunther$$b3$$eCorresponding author
001035293 773__ $$0PERI:(DE-600)3015727-4$$a10.1016/j.xcrp.2024.102340$$gVol. 5, no. 12, p. 102340 -$$n12$$p102340 - 102352$$tCell reports / Physical science$$v5$$x2666-3864$$y2024
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