Hauptseite > Publikationsdatenbank > Experimental correlation of anionic mass transport and lithium dendrite growth in solid-state polymer-based lithium metal batteries > print

001     1035293
005     20250224202208.0
024 7 _ |a 10.1016/j.xcrp.2024.102340
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100 1 _ |a Thienenkamp, Johannes H.
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245 _ _ |a Experimental correlation of anionic mass transport and lithium dendrite growth in solid-state polymer-based lithium metal batteries
260 _ _ |a [New York, NY]
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520 _ _ |a Various metal deposition models have been proposed for alkali metal batteries, but the experimental acces-sibility of designated driving forces and characteristics of specific morphologies is still limited. A combinedmethod portfolio comprising operando 1D 19 F MRI, in situ 7 Li NMR, and dynamic electrochemical impedancespectroscopy (EIS) experiments is presented. Experimental evidence of the relation of capacity-degradingdendritic Li metal growth and anionic mass-transport quantities beyond Sand’s time in polymer-based Limetal batteries is demonstrated. Comparison of anionic mass transport and morphological changes in Limetal in Li||Li and NMC 622||Li cells revealed that elevated anion drift velocities within electrolytes are corre-lated with pronounced dendrite growth. Higher cell voltages are associated with increased anion drift veloc-ities and hence dendrite growth, as reflected by a 2.5-fold increase in velocities in NMC 622||Li compared to Li||Li cells. This highlights the potential of the introduced method portfolio for experimental evaluation of poly-mer electrolytes and artificial coatings suitable for alkali metal batteries
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700 1 _ |a Lennartz, Peter
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700 1 _ |a Winter, Martin
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700 1 _ |a Brunklaus, Gunther
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773 _ _ |a 10.1016/j.xcrp.2024.102340
|g Vol. 5, no. 12, p. 102340 -
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