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@ARTICLE{Stroyuk:1037135,
      author       = {Stroyuk, Oleksandr and Raievska, Oleksandra and Hauch, Jens
                      and Brabec, Christoph J.},
      title        = {{A}tomically thin 2{D} materials for solution-processable
                      emerging photovoltaics},
      journal      = {Chemical communications},
      volume       = {61},
      number       = {3},
      issn         = {0022-4936},
      address      = {Cambridge},
      publisher    = {Soc.},
      reportid     = {FZJ-2025-00482},
      pages        = {455 - 475},
      year         = {2025},
      abstract     = {Atomically thin 2D materials, such as graphene and graphene
                      oxide, covalent organic frameworks, layered carbides, and
                      metal dichalcogenides, reveal a unique variability of
                      electronic and chemical properties, ensuring their prospects
                      in various energy generation, conversion, and storage
                      applications, including light harvesting in emerging
                      photovoltaic (ePV) devices with organic and perovskite
                      absorbers. Having an extremely high surface area, the 2D
                      materials allow a broad variability of the bandgap and
                      interband transition type, conductivity, charge carrier
                      mobility, and work function through mild chemical
                      modifications, external stimuli, or combination with other
                      2D species into van-der-Waals heterostructures. This review
                      provides an account of the most prominent “selling
                      points” of atomically thin 2D materials as components of
                      ePV solar cells, including highly tunable charge extraction
                      selectivity and work function, structure-directing and
                      stabilizing effects on halide perovskite light absorbers, as
                      well as broad adaptability of 2D materials to solution-based
                      manufacturing of ePV solar cells using sustainable and
                      upscalable printing technologies. A special focus is placed
                      on the large potential of the materials discovery and design
                      of ePV functionalities based on van-der-Waals stacking of
                      atomically thin 2D building blocks, which can open a vast
                      compositional domain of new materials navigable with
                      machine-learning-based accelerated materials screening},
      cin          = {IET-2},
      ddc          = {540},
      cid          = {I:(DE-Juel1)IET-2-20140314},
      pnm          = {1212 - Materials and Interfaces (POF4-121)},
      pid          = {G:(DE-HGF)POF4-1212},
      typ          = {PUB:(DE-HGF)16},
      pubmed       = {39641155},
      UT           = {WOS:001370799600001},
      doi          = {10.1039/D4CC05133E},
      url          = {https://juser.fz-juelich.de/record/1037135},
}