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001037614 1001_ $$00009-0005-7231-7204$$aKong, Mengqin$$b0
001037614 245__ $$aLead-Free Perovskite Cs 2 Ag x Na 1– x Bi y In 1– y Cl 6 Microcrystals for Scattering–Fluorescent Luminescent Solar Concentrators
001037614 260__ $$aWashington, DC$$bSoc.$$c2025
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001037614 520__ $$aIn recent years, luminescent solar concentrators (LSCs) have gained a renaissance as a pivotal transparent photovoltaic (PV) for building-integrated photovoltaics (BIPVs). However, most of the studies focused on light-selective LSCs, and less attention was paid to the utilization of the full solar spectrum. In this study, a lead-free microcrystal Cs2AgxNa1–xBiyIn1–yCl6 (CANBIC) perovskite phosphor is demonstrated to have bifunctional effects of luminescent down-shifting (LDS) and light scattering for the fabrication of LSCs, realizing light response from ultraviolet (UV) to NIR regions by an edge-mounted Si solar cell. The optimized CANBIC content (30 mg) in an LSC realizes the best optical efficiency (ηopt) of 5.40% and an average visible transmission (AVT) of >50%. This contributes to the improvement in short circuit current density (JSC) up to 1.232 mA/cm2 for the LSC–PV system (one-edge mounted Si solar cell) as a result of the best power conversion efficiencies (PCEs) of 0.463% and 1.852% for the LSC–PV and LSC–4PV systems (four-edge mounted Si solar cells), respectively. An Al foil is applied as a reflection background in the LSC–4PV system, and a champion PCE of 3.14% is realized due to an improved JSC of up to 7.94 mA/cm2 in total. Furthermore, the LSC maintains superior stability under exposure to continuous ultraviolet illumination or in ambient air.
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001037614 536__ $$0G:(DE-HGF)POF4-1214$$a1214 - Modules, stability, performance and specific applications (POF4-121)$$cPOF4-121$$fPOF IV$$x1
001037614 588__ $$aDataset connected to CrossRef, Journals: juser.fz-juelich.de
001037614 7001_ $$00000-0001-9098-9171$$aOsvet, Andres$$b1
001037614 7001_ $$aForberich, Karen$$b2
001037614 7001_ $$aBarabash, Anastasia$$b3
001037614 7001_ $$aErban, Christof$$b4
001037614 7001_ $$0P:(DE-HGF)0$$aBatentschuk, Miroslaw$$b5$$eCorresponding author
001037614 7001_ $$0P:(DE-Juel1)176427$$aBrabec, Christoph$$b6$$ufzj
001037614 773__ $$0PERI:(DE-600)2467494-1$$a10.1021/acsami.4c18315$$gVol. 17, no. 1, p. 1644 - 1653$$n1$$p1644 - 1653$$tACS applied materials & interfaces$$v17$$x1944-8244$$y2025
001037614 8564_ $$uhttps://juser.fz-juelich.de/record/1037614/files/lead-free-perovskite-cs2agxna1-xbiyin1-ycl6-microcrystals-for-scattering-fluorescent-luminescent-solar-concentrators.pdf$$yRestricted
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