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@INPROCEEDINGS{Hess:1037738,
author = {Hess, Steffen and Zhang, Shidong and Kadyk, Thomas and
Lehnert, Werner and Eikerling, Michael and Beale, Steven B.},
title = {{N}umerical {T}wo-{P}hase {S}imulations of {A}lkaline
{W}ater {E}lectrolyzers},
issn = {2151-2043},
reportid = {FZJ-2025-00898},
year = {2023},
abstract = {Alkaline water electrolyzers (AWE) have several advantages
over other types of electrolyzers, including their high
efficiency and especially their relatively low cost due to
the usage of non-precious metal catalysts, such as nickel
and iron, for the electrodes. Information about local
quantities and physical phenomena such as the formation of
gas bubbles, current densities, temperatures or local
species concentrations within a running cell are important
for their improvement. Multiphysical computational fluid
dynamics (CFD) simulations of electrochemical components
using detailed three-dimensional models can provide valuable
insight on local behaviors and characteristics that are
difficult or impossible to measure experimentally.This work
extends the CFD library openFuelCell21, which has been
implemented using the open-source platform OpenFOAM®, to
simulate AWE cells. The model considers the major transport
phenomena, including two-phase fluid flow, heat and mass
transfer, electrochemical reactions, species transfer and
charge transfer in the various functional regions of the
cell. It employs an Eulerian-Eulerian approach to
characterize the behavior of each phase comprising
interphase mass transport, momentum exchange and heat
transfer. Appropriate mapping functions are used to couple
the physically distinct regions together. A Butler-Volmer
equation characterizes the electrochemical reactions that
are assumed to occur in electrodes of finite thickness.This
model is used to simulate a single zero-gap AWE cell,
depicted in Fig. 1, for different operating conditions such
as varying temperatures and volumetric flow rates. The
conducted studies provide insight into the local formation
of the created gas phase (bubbles), the distribution of
species within the gas and electrolyte and their impact
towards the performance of the running cell. These
numerically obtained results are compared to in-house
available and gathered experimental data. Figure 1
demonstrates that the polarization curves obtained at
various temperatures are in good agreement with the
experimental data.},
month = {Oct},
date = {2023-10-08},
organization = {244th ECS Meeting, Gothenburg
(Sweden), 8 Oct 2023 - 12 Oct 2023},
cin = {IEK-14 / IET-4 / IET-3 / IET-1},
ddc = {540},
cid = {I:(DE-Juel1)IEK-14-20191129 / I:(DE-Juel1)IET-4-20191129 /
I:(DE-Juel1)IET-3-20190226 / I:(DE-Juel1)IET-1-20110218},
pnm = {1231 - Electrochemistry for Hydrogen (POF4-123)},
pid = {G:(DE-HGF)POF4-1231},
typ = {PUB:(DE-HGF)1},
doi = {10.1149/MA2023-02412016mtgabs},
url = {https://juser.fz-juelich.de/record/1037738},
}