001037877 001__ 1037877
001037877 005__ 20250203124524.0
001037877 0247_ $$2doi$$a10.1039/D4EE01647E
001037877 0247_ $$2ISSN$$a1754-5692
001037877 0247_ $$2ISSN$$a1754-5706
001037877 0247_ $$2datacite_doi$$a10.34734/FZJ-2025-01020
001037877 0247_ $$2WOS$$aWOS:001284318500001
001037877 037__ $$aFZJ-2025-01020
001037877 082__ $$a690
001037877 1001_ $$00000-0002-6018-5946$$aDong, Lirong$$b0
001037877 245__ $$aFully printed flexible perovskite solar modules with improved energy alignment by tin oxide surface modification
001037877 260__ $$aCambridge$$bRSC Publ.$$c2024
001037877 3367_ $$2DRIVER$$aarticle
001037877 3367_ $$2DataCite$$aOutput Types/Journal article
001037877 3367_ $$0PUB:(DE-HGF)16$$2PUB:(DE-HGF)$$aJournal Article$$bjournal$$mjournal$$s1738054654_3097
001037877 3367_ $$2BibTeX$$aARTICLE
001037877 3367_ $$2ORCID$$aJOURNAL_ARTICLE
001037877 3367_ $$00$$2EndNote$$aJournal Article
001037877 520__ $$aFully printed flexible perovskite solar cells (f-PSCs) show great potential for the commercialization of perovskite photovoltaics owing to their compatibility with high-throughput roll-to-roll (R2R) production. However, the challenge remains in the deficiency in controlling interfacial recombination losses of the functional layer, causing remarkable loss of power conversion efficiency (PCE) in industrial production. Here, a fullerene-substituted alkylphosphonic acid dipole layer is introduced between the R2R-printed tin oxide electron transport layer and the perovskite active layer to reduce the energetic barrier and to suppress surface recombination at the buried interface. The resulting f-PSCs exhibit a PCE of 17.0% with negligible hysteresis, retain 95% of their initial PCE over 3000 bending cycles and achieve a T95 lifetime of 1200 h under 1 sun and 65 °C in nitrogen atmosphere. Moreover, the fully printed flexible perovskite solar mini-modules (f-PSMs) with a 20.25 cm2 aperture area achieve a PCE of 11.6%. The encapsulated f-PSMs retain 90% of their initial PCE after 500 h damp-heat testing at 65 °C and 85% relative humidity (ISOS-D3). This work marks an important progress toward the realization of efficient and stable flexible perovskite photovoltaics for commercialization.
001037877 536__ $$0G:(DE-HGF)POF4-1214$$a1214 - Modules, stability, performance and specific applications (POF4-121)$$cPOF4-121$$fPOF IV$$x0
001037877 588__ $$aDataset connected to CrossRef, Journals: juser.fz-juelich.de
001037877 7001_ $$00000-0002-3005-5788$$aQiu, Shudi$$b1
001037877 7001_ $$00000-0002-7922-6824$$aGarcía Cerrillo, José$$b2
001037877 7001_ $$0P:(DE-Juel1)191164$$aWagner, Michael$$b3$$ufzj
001037877 7001_ $$aKasian, Olga$$b4
001037877 7001_ $$aFeroze, Sarmad$$b5
001037877 7001_ $$aJang, Dongju$$b6
001037877 7001_ $$00000-0002-8399-4244$$aLi, Chaohui$$b7
001037877 7001_ $$0P:(DE-Juel1)201923$$aM. Le Corre, Vincent$$b8
001037877 7001_ $$00000-0003-3468-3543$$aZhang, Kaicheng$$b9
001037877 7001_ $$00000-0002-9742-5800$$aPeisert, Heiko$$b10
001037877 7001_ $$00000-0003-1060-4003$$aU. Kosasih, Felix$$b11
001037877 7001_ $$00000-0003-3366-6442$$aDucati, Caterina$$b12
001037877 7001_ $$aArrive, Charline$$b13
001037877 7001_ $$0P:(DE-Juel1)200304$$aDU, Tian$$b14$$eCorresponding author$$ufzj
001037877 7001_ $$00000-0001-7673-8026$$aYang, Fu$$b15
001037877 7001_ $$0P:(DE-HGF)0$$aJ. Brabec, Christoph$$b16$$eCorresponding author
001037877 7001_ $$0P:(DE-Juel1)190193$$aEgelhaaf, Hans-Joachim$$b17
001037877 773__ $$0PERI:(DE-600)2439879-2$$a10.1039/D4EE01647E$$gVol. 17, no. 19, p. 7097 - 7106$$n19$$p7097 - 7106$$tEnergy & environmental science$$v17$$x1754-5692$$y2024
001037877 8564_ $$uhttps://juser.fz-juelich.de/record/1037877/files/d4ee01647e.pdf$$yOpenAccess
001037877 909CO $$ooai:juser.fz-juelich.de:1037877$$pdnbdelivery$$pdriver$$pVDB$$popen_access$$popenaire
001037877 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)191164$$aForschungszentrum Jülich$$b3$$kFZJ
001037877 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)201923$$aForschungszentrum Jülich$$b8$$kFZJ
001037877 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-Juel1)200304$$aForschungszentrum Jülich$$b14$$kFZJ
001037877 9101_ $$0I:(DE-588b)5008462-8$$6P:(DE-HGF)0$$aForschungszentrum Jülich$$b16$$kFZJ
001037877 9131_ $$0G:(DE-HGF)POF4-121$$1G:(DE-HGF)POF4-120$$2G:(DE-HGF)POF4-100$$3G:(DE-HGF)POF4$$4G:(DE-HGF)POF$$9G:(DE-HGF)POF4-1214$$aDE-HGF$$bForschungsbereich Energie$$lMaterialien und Technologien für die Energiewende (MTET)$$vPhotovoltaik und Windenergie$$x0
001037877 9141_ $$y2024
001037877 915__ $$0LIC:(DE-HGF)CCBY3$$2HGFVOC$$aCreative Commons Attribution CC BY 3.0
001037877 915__ $$0StatID:(DE-HGF)0200$$2StatID$$aDBCoverage$$bSCOPUS$$d2024-12-28
001037877 915__ $$0StatID:(DE-HGF)0160$$2StatID$$aDBCoverage$$bEssential Science Indicators$$d2024-12-28
001037877 915__ $$0StatID:(DE-HGF)1160$$2StatID$$aDBCoverage$$bCurrent Contents - Engineering, Computing and Technology$$d2024-12-28
001037877 915__ $$0StatID:(DE-HGF)1060$$2StatID$$aDBCoverage$$bCurrent Contents - Agriculture, Biology and Environmental Sciences$$d2024-12-28
001037877 915__ $$0StatID:(DE-HGF)0113$$2StatID$$aWoS$$bScience Citation Index Expanded$$d2024-12-28
001037877 915__ $$0StatID:(DE-HGF)0150$$2StatID$$aDBCoverage$$bWeb of Science Core Collection$$d2024-12-28
001037877 915__ $$0StatID:(DE-HGF)0510$$2StatID$$aOpenAccess
001037877 915__ $$0StatID:(DE-HGF)1150$$2StatID$$aDBCoverage$$bCurrent Contents - Physical, Chemical and Earth Sciences$$d2024-12-28
001037877 915__ $$0StatID:(DE-HGF)0430$$2StatID$$aNational-Konsortium$$d2024-12-28$$wger
001037877 915__ $$0StatID:(DE-HGF)0300$$2StatID$$aDBCoverage$$bMedline$$d2024-12-28
001037877 915__ $$0StatID:(DE-HGF)0199$$2StatID$$aDBCoverage$$bClarivate Analytics Master Journal List$$d2024-12-28
001037877 920__ $$lyes
001037877 9201_ $$0I:(DE-Juel1)IET-2-20140314$$kIET-2$$lHelmholtz-Institut Erlangen-Nürnberg Erneuerbare Energien$$x0
001037877 980__ $$ajournal
001037877 980__ $$aVDB
001037877 980__ $$aUNRESTRICTED
001037877 980__ $$aI:(DE-Juel1)IET-2-20140314
001037877 9801_ $$aFullTexts