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@ARTICLE{Cui:1038133,
author = {Cui, Jinchao and Zhang, Jiyun and Jing, Jingyi and Wang, Ya
and Du, Gaohui and Yang, Yongzhen and Yan, Lingpeng and Su,
Qingmei},
title = {{A}dvances in {I}n {S}itu {TEM} for {D}ynamic {S}tudies of
{C}arbon‐{B}ased {A}nodes in {A}lkali {M}etal‐{I}on
{B}atteries},
journal = {Advanced functional materials},
volume = {35},
number = {13},
issn = {1616-301X},
address = {Weinheim},
publisher = {Wiley-VCH},
reportid = {FZJ-2025-01180},
pages = {2418059},
year = {2025},
abstract = {High-energy-density anode materials are crucial for
achieving high performance alkali metal-ion batteries
(AMIBs). In situ transmission electron microscopy (TEM)
enables real-time observation of microstructural changes in
electrode materials and interfaces during
charging/discharging, crucial for designing high-performance
anodes. This paper highlights and reviews the dynamic
studies of the relationship between the structure and the
electrochemical performance of carbon-based composite
materials used as anodes in AMIBs by in situ TEM. First, the
in situ TEM technique and cell construction method are
introduced, followed by an overview of in situ TEM
integrates with other advanced measurement techniques.
Second, the fundamental working principles of various AMIBs
and the energy storage mechanisms of anode materials are
explained, along with the achievable functions of in situ
TEM in AMIBs. Third, from different carbon matrix
structures, including carbon-supported, carbon-embedded,
carbon-coated, carbon-encapsulated, and hybrid
carbon-composite structures, in situ dynamic studies on the
electrochemical behaviors of these carbon-based anode
materials by TEM are covered in depth. Finally, a summary of
the design ideas and the technical application of in situ
TEM for carbon-based anode composites is provided, followed
by a suggestion for current challenges and future research
paths.},
cin = {IET-2},
ddc = {530},
cid = {I:(DE-Juel1)IET-2-20140314},
pnm = {1212 - Materials and Interfaces (POF4-121) / 1214 -
Modules, stability, performance and specific applications
(POF4-121)},
pid = {G:(DE-HGF)POF4-1212 / G:(DE-HGF)POF4-1214},
typ = {PUB:(DE-HGF)36 / PUB:(DE-HGF)16},
UT = {WOS:001362709400001},
doi = {10.1002/adfm.202418059},
url = {https://juser.fz-juelich.de/record/1038133},
}