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001038552 1001_ $$0P:(DE-Juel1)178670$$aStroyuk, Oleksandr$$b0$$eCorresponding author
001038552 245__ $$aExperimental design of (Cs,Rb) 2 Sn(Bi)Cl 6 blue phosphors by cation-substitution-induced lattice strain
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001038552 520__ $$aA mild high-throughput synthesis of doubly substituted (CsxRb1−x)2SnyBi1−yCl6 perovskites yields single-phase solid-solution compounds in the compositional domain of x = 0–1 and y ≥ 0.75. Bi-substituted compounds emit relatively intense and broadband blue photoluminescence (PL) peaked at 455 nm, originating from the self-trapped excitonic states. Both Sn/Bi and Cs/Rb substitutions were found to exert a lattice strain with the maximal strain magnitudes observed close to x = 0.5 and y = 0.90. The PL parameters of the single-phase (CsxRb1−x)2SnyBi1−yCl6 samples, in particular, the PL intensity and lifetime, as well as the rate constants of radiative and non-radiative recombination, correlate with the strain magnitude.
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001038552 7001_ $$0P:(DE-Juel1)188483$$aRaievska, Oleksandra$$b1$$ufzj
001038552 7001_ $$0P:(DE-HGF)0$$aDaum, Manuel$$b2
001038552 7001_ $$0P:(DE-Juel1)200347$$aKupfer, Christian$$b3$$ufzj
001038552 7001_ $$aOsvet, Andres$$b4
001038552 7001_ $$0P:(DE-Juel1)177626$$aHauch, Jens$$b5$$ufzj
001038552 7001_ $$0P:(DE-Juel1)176427$$aBrabec, Christoph$$b6$$ufzj
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001038552 8564_ $$uhttps://juser.fz-juelich.de/record/1038552/files/Sn_LFPs_paper_revision2.pdf$$yPublished on 2024-12-02. Available in OpenAccess from 2025-12-02.
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