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@ARTICLE{Ahrens:1039732,
author = {Ahrens, Lara and Mikulics, Martin and Schröder, Steffen
and Mayer, Joachim and Hardtdegen, Hilde Helen},
title = {{L}aser-{M}icro-{A}nnealing of {M}icrocrystalline
{N}i-{R}ich {NCM} {O}xide: {T}owards {M}icro-{C}athodes
{I}ntegrated on {P}olyethylene {T}erephthalate {F}lexible
{S}ubstrates},
journal = {Materials},
volume = {18},
number = {3},
issn = {1996-1944},
address = {Basel},
publisher = {MDPI},
reportid = {FZJ-2025-01776},
pages = {680 -},
year = {2025},
note = {This research was funded by the Joint Lab for Integrated
Model and Data-Driven Material Characterization (MDMC) of
the Helmholtz Association.},
abstract = {Here in this work, we report on micro-Raman spectroscopy
investigations performed on freestanding Ni-rich NCM
(LixNi0.83Co0.11Mn0.06O2) microcrystals transferred to
flexible polyethylene terephthalate (PET) host substrates.
This technological procedure introduces a first building
block for future on-chip-integrated micro-accumulators for
applications in flexible optoelectronics, sensors,
microbiology, and human medicine. An after-synthesis thermal
treatment was used to help improve the material homogeneity
and perfection of the cathode material. To this end, a local
laser micro-annealing process was applied to the
freestanding Ni-rich NCM microcrystals. The thermally
initialized structural processes in the singular
micro-cathode units were characterized and determined by
micro-Raman spectroscopy. Micro-Raman mapping images
revealed the evolution of a recrystallization process after
the local annealing procedure. Furthermore, laser
micro-annealing led to the suppression of the pristine
“polycrystalline morphology” of the investigated
micro-cathode regions. Besides the dominant characteristic
Raman mode at ~1085 cm−1, most likely ascribed to lithium
carbonate, metal oxides with Raman modes around ~550 cm−1
were identified. This highly efficient transfer and
integration technology represents a basic building block
towards micrometer-sized accumulators for a large range of
emerging applications.},
cin = {ER-C-2},
ddc = {600},
cid = {I:(DE-Juel1)ER-C-2-20170209},
pnm = {5353 - Understanding the Structural and Functional Behavior
of Solid State Systems (POF4-535)},
pid = {G:(DE-HGF)POF4-5353},
typ = {PUB:(DE-HGF)16},
pubmed = {39942346},
UT = {WOS:001420208300001},
doi = {10.3390/ma18030680},
url = {https://juser.fz-juelich.de/record/1039732},
}