Hauptseite > Publikationsdatenbank > Paramagnetic fluctuations of the magnetocaloric compound MnFe 4 Si 3 > print |
001 | 1039787 | ||
005 | 20250414120451.0 | ||
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100 | 1 | _ | |a Biniskos, Nikolaos |0 P:(DE-Juel1)180764 |b 0 |e Corresponding author |
245 | _ | _ | |a Paramagnetic fluctuations of the magnetocaloric compound MnFe 4 Si 3 |
260 | _ | _ | |a Woodbury, NY |c 2025 |b Inst. |
336 | 7 | _ | |a article |2 DRIVER |
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520 | _ | _ | |a An inelastic neutron scattering technique is employed to investigate the paramagnetic spin dynamics in a single-crystalline sample of the magnetocaloric compound MnFe4Si3. In the investigated temperature range, 1.033 x TC to 1.5 x TC , where TC is the Curie temperature, the spin fluctuations are well described by the ferromagnetic Heisenberg model predictions. Apart from the Heisenberg exchange, additional pseudodipolar interactions manifest through a finite long-wavelength relaxation rate that vanishes at the transition temperature (TC = 305 K). Based on the characteristic extent of spin fluctuations in wave-vector and energy space, we determine that the nature of magnetism in MnFe4Si3 is localized above room temperature. This contrasts with the most celebrated Mn- and Fe-based magnetocaloric materials that are considered as itinerant magnets. The field dependence of the paramagnetic spectra shows a strong suppression of the quasielastic excitations, while a field-induced spin-wave mode appears at finite-energy transfers for a magnetic field of 2 T. This modification of the spectra suggests a decrease of magnetic entropy with applied magnetic field that finds echo in the magnetocaloric properties of the system. |
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700 | 1 | _ | |a Raymond, S. |0 0000-0002-5421-5061 |b 3 |
773 | _ | _ | |a 10.1103/PhysRevB.111.054424 |g Vol. 111, no. 5, p. 054424 |0 PERI:(DE-600)2844160-6 |n 5 |p 054424 |t Physical review / B |v 111 |y 2025 |x 2469-9950 |
856 | 4 | _ | |y OpenAccess |u https://juser.fz-juelich.de/record/1039787/files/PhysRevB.111.054424.pdf |
856 | 4 | _ | |y OpenAccess |u https://juser.fz-juelich.de/record/1039787/files/manuscript_after_review.pdf |
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