Home > Publications database > Bottom-up Synthesis and Characterization of Porous 12-Atom-Wide Armchair Graphene Nanoribbons > print

001     1040277
005     20250310131246.0
024 7 _ |a 10.1021/acs.nanolett.4c01106
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100 1 _ |a Fan, Qitang
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245 _ _ |a Bottom-up Synthesis and Characterization of Porous 12-Atom-Wide Armchair Graphene Nanoribbons
260 _ _ |a Washington, DC
|c 2024
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520 _ _ |a Although several porous carbon/graphene nanorib-bons (GNRs) have been prepared, a direct comparison of theelectronic properties between a nonporous GNR and itsperiodically perforated counterpart is still missing. Here, we reportthe synthesis of porous 12-atom-wide armchair-edged GNRs froma bromoarene precursor on a Au(111) surface via hierarchicalUllmann and dehydrogenative coupling. The selective formation ofporous 12-GNRs was achieved through thermodynamic andkinetic reaction control combined with tailored precursor design.The structure and electronic properties of the porous 12-GNRwere elucidated by scanning tunneling microscopy/spectroscopyand density functional theory calculations, revealing that the poresinduce a 2.17 eV band gap increase compared to the nonporous12-AGNR on the same surface.
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700 1 _ |a Ruan, Zilin
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700 1 _ |a Werner, Simon
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700 1 _ |a Naumann, Tim
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700 1 _ |a Bolat, Rustem
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700 1 _ |a Martinez-Castro, Jose
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700 1 _ |a Koehler, Tabea
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700 1 _ |a Vollgraff, Tobias
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700 1 _ |a Hieringer, Wolfgang
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700 1 _ |a Mandalia, Raviraj
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700 1 _ |a Neiß, Christian
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700 1 _ |a Görling, Andreas
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700 1 _ |a Tautz, F. Stefan
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700 1 _ |a Sundermeyer, Jörg
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700 1 _ |a Gottfried, J. Michael
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773 _ _ |a 10.1021/acs.nanolett.4c01106
|g Vol. 24, no. 35, p. 10718 - 10723
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