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| Hauptseite > Publikationsdatenbank > Comparative Study of Iminodibenzyl and Diphenylamine Derivatives as Hole Transport Materials in Inverted Perovskite Solar Cells > print |
| Hauptseite > Publikationsdatenbank > Comparative Study of Iminodibenzyl and Diphenylamine Derivatives as Hole Transport Materials in Inverted Perovskite Solar Cells > print |
| 001 | 1040384 | ||
| 005 | 20250414120448.0 | ||
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| 100 | 1 | _ | |a Caicedo-Reina, Mauricio |0 0000-0002-0014-0041 |b 0 |
| 245 | _ | _ | |a Comparative Study of Iminodibenzyl and Diphenylamine Derivatives as Hole Transport Materials in Inverted Perovskite Solar Cells |
| 260 | _ | _ | |a Weinheim |c 2025 |b Wiley-VCH |
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| 520 | _ | _ | |a Perovskite solar cells (PSCs) have recently achieved over 26 % power conversion efficiency, challenging the dominance of silicon-based alternatives. This progress is significantly driven by innovations in hole transport materials (HTMs), which notably influence the efficiency and stability of PSCs. However, conventional organic HTMs like Spiro-OMeTAD and PTAA, although highly efficient, suffer from thermal degradation, moisture ingress, and high cost. This study explores the potential of iminodibenzyl, a moiety known for its strong electron-donating capabilities in pharmaceutical applications, as a novel HTM. A series of fluorene-based derivatives incorporating iminodibenzyl (TMF-2 and TDF-2) and diphenylamine (TMF-1 and TDF-1) units were synthesized and characterized. The new HTMs demonstrated commendable optical, electrochemical, and thermal properties, as well as enhanced photostability. Among them, TDF-2 achieved a power conversion efficiency (PCE) of 19.38 %, the highest of the new materials. Although these efficiencies are slightly lower than the benchmark PTAA (20.20 %), the study underscores the potential of iminodibenzyl to enhance photostability and increase HOMO levels, making it a promising candidate for future HTM development in PSCs. |
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| 700 | 1 | _ | |a Rocha-Ortiz, Juan S. |0 P:(DE-Juel1)201567 |b 1 |e Corresponding author |
| 700 | 1 | _ | |a Wu, Jianchang |0 P:(DE-Juel1)192542 |b 2 |
| 700 | 1 | _ | |a Bornschlegl, Andreas J. |0 0000-0001-9992-5449 |b 3 |
| 700 | 1 | _ | |a Leon, Salvador |0 0000-0002-2757-9417 |b 4 |
| 700 | 1 | _ | |a Barabash, Anastasia |0 0000-0003-1732-1233 |b 5 |
| 700 | 1 | _ | |a Dario Perea, Jose |0 0000-0001-7669-7797 |b 6 |
| 700 | 1 | _ | |a Wang, Yunuo |b 7 |
| 700 | 1 | _ | |a Arango-Marín, Vanessa |0 0000-0001-9797-8280 |b 8 |
| 700 | 1 | _ | |a Ortiz, Alejandro |0 0000-0002-4392-9456 |b 9 |
| 700 | 1 | _ | |a Lüer, Larry |b 10 |
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| 700 | 1 | _ | |a Insuasty, Braulio |b 12 |
| 700 | 1 | _ | |a Brabec, Christoph |0 P:(DE-Juel1)176427 |b 13 |e Corresponding author |u fzj |
| 773 | _ | _ | |a 10.1002/chem.202404251 |g p. e202404251 |0 PERI:(DE-600)1478547-X |n 13 |p e202404251 |t Chemistry - a European journal |v 31 |y 2025 |x 0947-6539 |
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