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@ARTICLE{Lebendig:1040455,
author = {Lebendig, Florian and Müller, Michael},
title = {{I}nfluence of {B}iofuel {B}lending on {I}norganic
{C}onstituent {B}ehavior and {I}mpact in {F}luidized-{B}ed
{G}asification},
journal = {Energy $\&$ fuels},
volume = {39},
number = {8},
issn = {0887-0624},
address = {Columbus, Ohio},
publisher = {American Chemical Society},
reportid = {FZJ-2025-01907},
pages = {3868 - 3881},
year = {2025},
abstract = {A promising technology for producing carbon-neutral fuels
is fluidized-bed gasification of biomass. In combination
with chemical looping gasification (CLG), the process
becomes even more efficient. However, using biomass-based
fuels can lead to significant ash-related issues, including
bed agglomeration, fouling, deposition, slagging, and
high-temperature corrosion. To address these issues, several
biomass upgrading approaches are used to improve the quality
of the feedstock for gasification. These approaches include
torrefaction, water leaching, and blending with different
additives. This study focuses on the influence of additives
and biomass co-blending with low-cost biofuels on the
behavior of inorganic constituents and under
gasification-like conditions at 950 °C and the
corresponding impact in fluidized-bed gasification. For
example, blending (upgraded) barley straw with 2 wt $\%$
CaCO3 resulted in a decrease in slag and a corresponding
increase in the proportion of solid oxides. This indicates
that thermal stability can be expected at operating
temperatures up to 950 °C. Similarly, adding Ca/Si-rich
biowaste components increases the ash softening point of
herbaceous biofuels. Furthermore, the results show that
adding Ca-based or woody biofuel components has a chemical
effect on the fate of volatile inorganics. For example,
increasing the concentration of calcium in the fuel
significantly reduces the release of HCl and partially
reduces the release of sulfur species, thus reducing the
corrosion risk. These results contribute to the development
of more efficient and cleaner biomass gasification processes
for producing carbon-neutral fuels.},
cin = {IMD-1},
ddc = {660},
cid = {I:(DE-Juel1)IMD-1-20101013},
pnm = {1241 - Gas turbines (POF4-124) / CLARA - Chemical Looping
gAsification foR sustainAble production of biofuels
(817841)},
pid = {G:(DE-HGF)POF4-1241 / G:(EU-Grant)817841},
typ = {PUB:(DE-HGF)16},
pubmed = {40040731},
UT = {WOS:001433736000001},
doi = {10.1021/acs.energyfuels.4c05818},
url = {https://juser.fz-juelich.de/record/1040455},
}